Magnetic and electronic Co states in layered cobaltate GdBaCo2O5.5-x

M. Garcia-Fernandez; V. Scagnoli; U. Staub; A. M. Mulders; M. Janousch; Y. Bodenthin; D. Meister; B. D. Patterson; A. Mirone; Y. Tanaka; T. Nakamura; S. Grenier; Y. Huang; K. Conder

doi:10.1103/physrevb.78.054424

arXiv · 0808.1681

Magnetic and electronic Co states in layered cobaltate GdBaCo2O5.5-x

M. Garcia-Fernandez·V. Scagnoli·U. Staub·A. M. Mulders·M. Janousch·Y. Bodenthin·D. Meister·B. D. Patterson·A. Mirone·Y. Tanaka·T. Nakamura·S. Grenier·Y. Huang·K. Conder

View original source ↗Read source document ↗Export metadata ↓

Abstract

We have performed non-resonant x-ray diffraction, resonant soft and hard x-ray magnetic diffraction, soft x-ray absorption and x-ray magnetic circular dichroism measurements to clarify the electronic and magnetic states of the Co3+ ions in GdBaCo2O5.5. Our data are consistent with a 3+ Py Co HS state at the pyramidal sites and a 3+ Oc Co LS state at the octahedral sites. The structural distortion, with a doubling of the a axis (2ap x 2ap x 2ap cell), shows alternating elongations and contractions of the pyramids and indicates that the metal-insulator transition is associated with orbital order in the t2g orbitals of the 3+ Py Co HS state. This distortion corresponds to an alternating ordering of xz and yz orbitals along the a and c axes for the 3+ Py Co . The orbital ordering and pyramidal distortion lead to deformation of the octahedra, but the 3+ Oc Co LS state does not allow an orbital order to occur for the 3+ Oc Co ions. The soft x-ray magnetic diffraction results indicate that the magnetic moments are aligned in the ab plane but are not parallel to the crystallographic a or b axes. The orbital order and the doubling of the magnetic unit cell along the c axis support a non-collinear magnetic structure. The x-ray magnetic circular dichroism data indicate that there is a large orbital magnetic contribution to the total ordered Co moment.

Explore related subjects

cond-mat.str-el

Keep this discovery

Explore connections, maps & timelines

BibTeX RIS

M. Garcia-Fernandez, V. Scagnoli, U. Staub, A. M. Mulders, M. Janousch, Y. Bodenthin, D. Meister, B. D. Patterson, A. Mirone, Y. Tanaka, T. Nakamura, S. Grenier, Y. Huang, K. Conder. 2008-08-12. Magnetic and electronic Co states in layered cobaltate GdBaCo2O5.5-x. https://doi.org/10.1103/physrevb.78.054424

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

arXiv2026

Collective excitations in chiral spin liquid: chiral roton and long-wavelength nematic mode

Chiral spin liquid (CSL) is a magnetic analogue of the fractional quantum Hall (FQH) liquid. Collective excitations play a vital role in shaping our understanding of these exotic quantum phases of matter and their quantum phase transitions. While the magneto-roton and long-wavelength chiral graviton modes in the FQH and fractional Chern insulator (FCI) liquids have been extensively explored, whether CSLs host analogous or qualitatively different modes remains elusive. Here we explore the collective excitations in the SU(2) symmetric CSL phase. Combining exact diagonalization and time-dependent variational principle calculations, we identify two spin-singlet collective modes: a chiral p-wave roton mode at finite momentum, and a elliptically polarized d-wave nematic mode at zero momentum, both of which are prominent across the CSL phase. The chiral p-wave singlet roton has no counterpart in FQH of FCI systems, and the q = 0 d-wave mode also exhibits fingerprint distinct from those of FQH/FCI liquids. We also elucidate that both singlet modes are general for CSLs on various lattice models. By tuning J2, we find the nematic mode to be pronouncedly soft, together with the spin-triplet two-spinon bound states, potentially promoting strong nematic and spin stripe instabilities. Our work paves the way for further understanding CSL from the dynamical perspective and provides new spectroscopic signatures for future experiments of CSL candidates.

cond-mat.str-el↗

arXiv2026

Extracting central charge from ground-state overlaps of spatially deformed Hamiltonians

We show that the conformal anomaly of a $(1+1)$-dimensional conformal field theory can be extracted directly from a ground-state wave-function overlap associated with a spatial conformal deformation. Focusing on the $q$-Möbius deformation, we derive an exact overlap formula between the deformed and undeformed ground states, whose exponent directly encodes the central charge. Motivated by this result, we construct a lattice estimator based solely on ground-state overlaps and apply it to representative critical quantum chains and the gapless edge modes of a two-dimensional Chern insulator. Numerical results demonstrate that the resulting overlaps provide a simple and robust probe of the central charge in microscopic models. We further demonstrate that the deformed ground states retain universal geometric structures in their entanglement spectra and entanglement entropies. These results provide a simple wave-function-based route to probing conformal data in critical systems and topological edge modes.

cond-mat.str-el↗

arXiv2026

Propagation and localization of spin excitations at altermagnetic domain walls

Altermagnets (A$\ell$Ms) are spin-compensated materials in which opposite-spin sublattices are connected by a symmetry that causes a spin splitting in their elementary excitations. As there is a strong effect of altermagnetism on domain wall properties, it is quite natural to also expect an enrichment of the physics of magnetic excitations at A$\ell$M domain walls. Here, we consider the propagation of spin eigen-excitations along domain walls in easy-axial $d$-wave A$\ell$Ms. Investigating the presence of bound states localized on a domain wall, we find that the effect of the A$\ell$M on the bound states strongly depends on the orientation of the domain wall relative to the crystallographic directions. If the domain wall is oriented along a nodal direction [100] or [010], A$\ell$M does not change the number of bound states; however, it leads to a nonlinear dispersion and a tilt of the wavefront. The effect of A$\ell$M is strongest when the domain wall is oriented along the directions [110] or [$\bar{1}$10], i.e., along the directions of the strongest A$\ell$M splitting in the magnon spectrum. In this case, (i) the additional gapped bound states appear, (ii) degeneracy of the eigenstates with respect to their polarization (right-handed or left-handed precession of the N{é}el vector) is removed, and (iii) the localization area of the bound states strongly depends on the eigenfrequency. The latter may lead to strong localization of the bound state at the domain wall. We further consider the influence of a static magnetic field that is applied along the easy axis, and find that the magnetic field induces an asymmetry between the localization regions on opposite sides of the domain wall and sets an upper limit on the absolute value of the propagating eigenstate's wave vector.

cond-mat.str-el↗