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arXiv · 0809.1248

New structural and magnetic aspects of the nanotube system Na2V3O7

O. Zaharko·J. L. Gavilano·Th. Straessle·C. F. Miclea·A. C. Mota·Y. Filinchuk·D. Chernyshov·P. P. Deen·B. Rahaman·T. Saha-Dasgupta·R. Valenti'·Y. Matsushita·A. Doenni·H. Kitazawa
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Abstract

We present new experimental results of low temperature x-ray synchrotron diffraction, neutron scattering and very low temperature (mK-range) bulk measurements on the nanotube system ${\tube}$. The crystal structure determined from our data is similar to the previously proposed model (P. Millet {\it et al.} J. Solid State Chem. $\bf{147}$, 676 (1999)), but also deviates from it in significant details. The structure comprises nanotubes along the c-axis formed by stacking units of two V-rings buckled in the $ab$-plane. The space group is P$\bar{3}$ and the composition is nonstoichiometric, Na(2-x)V3O7, x=0.17. The thermal evolution of the lattice parameters reveals anisotropic lattice compression on cooling. Neutron scattering experiments monitor a very weak magnetic signal at energies from -20 to 9 meV. New magnetic susceptibility, specific heat measurements and decay of remanent magnetization in the 30 mK - 300 mK range reveal that the previously observed transition at ~76 mK is spin-glass like with no long-range order. Presented experimental observations do not support models of isolated clusters, but are compatible with a model of odd-legged S=1/2 spin tubes possibly segmented into fragments with different lengths.

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O. Zaharko, J. L. Gavilano, Th. Straessle, C. F. Miclea, A. C. Mota, Y. Filinchuk, D. Chernyshov, P. P. Deen, B. Rahaman, T. Saha-Dasgupta, R. Valenti', Y. Matsushita, A. Doenni, H. Kitazawa. 2008-09-07. New structural and magnetic aspects of the nanotube system Na2V3O7. https://doi.org/10.1103/physrevb.78.214426

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