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arXiv · 1106.2706

Two-magnon Raman scattering in A$_{0.8}$Fe$_{1.6}$Se$_2$ systems: competition between superconductivity and antiferromagnetic order

A. M. Zhang·J. H. Xiao·Y. S. Li·J. B. He·D. M. Wang·G. F. Chen·B. Normand·Q. M. Zhang·T. Xiang
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Abstract

We have performed Raman-scattering measurements on high-quality single crystals of A$_{0.8}$Fe$_{1.6}$Se$_2$ superconductors of several compositions. We find a broad, asymmetric peak around 1600 cm$^{-1}$ (200 meV), which we identify as a two-magnon process involving optical magnons. The intensity of the two-magnon peak falls sharply on entering the superconducting phase. This effect, which is entirely absent in the non-superconducting system KFe$_{1.5}$Se$_2$, requires a strong mutual exclusion between antiferromagnetism and superconductivity arising from proximity effects within regions of microscale phase separation.

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A. M. Zhang, J. H. Xiao, Y. S. Li, J. B. He, D. M. Wang, G. F. Chen, B. Normand, Q. M. Zhang, T. Xiang. 2011-06-14. Two-magnon Raman scattering in A$_{0.8}$Fe$_{1.6}$Se$_2$ systems: competition between superconductivity and antiferromagnetic order. https://doi.org/10.1103/physrevb.85.214508

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