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arXiv · 1108.1297

Magnons and electromagnons in a spin-lattice-coupled frustrated magnet CuFeO2 as seen via inelastic neutron scattering

Taro Nakajima·Azusa Suno·Setsuo Mitsuda·Noriki Terada·Shojiro Kimura·Koji Kaneko·Hiroki Yamauchi
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Abstract

We have investigated spin-wave excitations in a four-sublattice (4SL) magnetic ground state of a frustrated magnet CuFeO2, in which `electromagnon' (electric-field-active magnon) excitation has been discovered by recent terahertz time-domain spectroscopy [Seki et al. Phys. Rev. Lett. 105 097207 (2010)]. In previous study, we have identified two spin-wave branches in the 4SL phase by means of inelastic neutron scattering measurements under applied uniaxial pressure. [T. Nakajima et al. J. Phys. Soc. Jpn. 80 014714 (2011) ] In the present study, we have performed high-energy-resolution inelastic neutron scattering measurements in the 4SL phase, resolving fine structures of the lower-energy spin-wave branch near the zone center. Taking account of the spin-driven lattice distortions in the 4SL phase, we have developed a model Hamiltonian to describe the spin-wave excitations. The determined Hamiltonian parameters have successfully reproduced the spin-wave dispersion relations and intensity maps obtained in the inelastic neutron scattering measurements. The results of the spin-wave analysis have also revealed physical pictures of the magnon and electromagnon modes in the 4SL phase, suggesting that collinear and noncollinear characters of the two spin-wave modes are the keys to understand the dynamical coupling between the spins and electric dipole moments in this system.

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Taro Nakajima, Azusa Suno, Setsuo Mitsuda, Noriki Terada, Shojiro Kimura, Koji Kaneko, Hiroki Yamauchi. 2011-08-05. Magnons and electromagnons in a spin-lattice-coupled frustrated magnet CuFeO2 as seen via inelastic neutron scattering. https://doi.org/10.1103/physrevb.84.184401

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