Quantum-statistical theory of Raman scattering processes

Adam Miranowicz; Stanislaw Kielich

Home/Archive/arXiv

arXiv · 1110.4959

Quantum-statistical theory of Raman scattering processes

Adam Miranowicz·Stanislaw Kielich

View original source ↗Read source document ↗Export metadata ↓

Abstract

Raman scattering from a great number of phonon modes is described from a quantum-statistical point of view within the standing-wave model. The master equation for the completely quantum case, including laser pump depletion and stochastic coupling of Stokes and anti-Stokes modes, is derived and converted to classical equations: either into a generalized Fokker-Planck equation and an equation of motion for the characteristic function or into the master equation in Fock representation. These two approaches are developed both in linear and nonlinear regime. A detailed analysis of scattering into Stokes and anti-Stokes modes in linear regime, i.e., under parametric approximation, is presented. The existence of s-parametrized quasiprobability distributions, in particular the Glauber-Sudarshan P-function, is investigated. An analysis of Raman scattering into separate Stokes and anti-Stokes modes in nonlinear regime, thus including pump depletion, is given. The master equation in Fock representation is solved exactly for the complete density matrix using the Laplace transform method. Short-time solutions, steady-state solutions and approximate compact form solutions are obtained. Relations between the quasidistribution approach based on the Fokker-Planck equation and the density matrix approach based on the master equation in Fock representation are presented. The photocount distribution and its factorial moments as well as variances and extremal variances of quadratures are calculated in both approaches giving the basis for the analysis of the quantum properties of radiation such as sub-Poissonian photon-counting statistics and squeezing. Various statistical moments obtained from numerical calculations utilizing our exact solutions, from the approximate relations for short times, and those obtained under parametric approximation are compared.

Explore related subjects

quant-ph

Keep this discovery

Explore connections, maps & timelines

BibTeX RIS

Adam Miranowicz, Stanislaw Kielich. 2011-10-22. Quantum-statistical theory of Raman scattering processes. https://arxiv.org/abs/1110.4959

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

arXiv2026

Quantum Authenticated Key Expansion with Key Recycling

Data privacy and authentication are two main security requirements for remote access and cloud services. While QKD has been explored to address data privacy concerns, oftentimes its use is separate from the client authentication protocol despite implicitly providing authentication. Here, we present a quantum authentication key expansion (QAKE) protocol that (1) integrates both authentication and key expansion within a single protocol, and (2) provides key recycling property - allowing all authentication keys to be reused. We analyse the security of the protocol in a QAKE framework adapted from a classical authentication key exchange (AKE) framework, providing separate security conditions for authentication and data privacy. We experimentally implemented the protocol with appropriate post-selection. Additional results on the security of pseudorandom basis generation in QAKE and decoy state BB84 are provided.

quant-ph↗

arXiv2026

Entanglement as Difference: Reduction-induced Minimal Partial Entropy Difference

Bipartite mixed-state quantum entanglement (QE) and its measures play a crucial role in both theoretical research and practical quantum applications. Its internal structure is far more complex and less well understood compared with bipartite pure-state QE. Some existing measures involve inherently intractable global optimizations, while others are only applicable to highly limited-dimensional quantum systems. Here based on the inherent feature that bipartite QE systems nonseparable necessarily implies that local reduced density matrix differs from its \textquotedblleft native\textquotedblright density matrix, we propose a more physical and intuitive measure termed Reduction-induced Minimal Partial Entropy Difference to quantify arbitrary bipartite mixed-state QE. Partial Von Neumann Entropy is only a pure-state special case of this method. This measure offers intrinsic structural %perspective insights into bipartite QE characterization, thereby establishing itself as a valuable complementary measure. Its intuitive and clear physical picture, combined with relatively low computational complexity and wide applicability, facilitates exploring its potential quantum information applications, hence its conceptual framework and line of thought deserve to be further developed to describe and quantify multipartite QE in the future.

quant-ph↗

arXiv2026

Non-local mass superpositions and optical clock interferometry in atomic ensemble quantum networks

Quantum networks are emerging as powerful platforms for sensing, communication, and fundamental tests of physics. We propose a programmable quantum sensing network based on entangled atomic ensembles, where optical clock qubits realize mass superpositions arising via mass-energy equivalence, as in atom and atom-clock interferometry. Our approach uniquely combines scalability to large atom numbers with minimal control requirements, relying only on collective addressing of internal atomic states. This enables the creation of both non-local and local superpositions with spatial separations beyond those achievable in conventional matter-wave interferometry with single atoms. Starting from Bell-type seed states distributed via photonic channels, collective operations within atomic ensembles coherently build many-body mass superpositions sensitive to gravitational redshift. The resulting architecture implements a non-local Ramsey interferometer, where gravitationally induced phase shifts are imprinted on non-local entangled states and are read out through local measurements at the network nodes. Beyond extending the spatial reach of mass superpositions, our scheme establishes a scalable, programmable platform to probe the interface of quantum mechanics and gravity, and offers a new experimental pathway to test atom and atom-clock interferometer proposals, e.g. for probing gravitational dephasing, in a network-based quantum laboratory.

quant-ph↗