Phase Space Approach to Laser-driven Electronic Wavepacket Propagation

Norio Takemoto; Asaf Shimshovitz; David J. Tannor

doi:10.1063/1.4732306

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arXiv · 1205.4449

Phase Space Approach to Laser-driven Electronic Wavepacket Propagation

Norio Takemoto·Asaf Shimshovitz·David J. Tannor

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Abstract

We propose a phase space method to propagate a quantum wavepacket driven by a strong external field. The method employs the so-called biorthogonal von Neumann basis recently introduced for the calculation of the energy eigenstates of time-independent quantum systems [A. Shimshovitz and D.J. Tannor, arXiv:1201.2299v1]. While the individual elements in this basis set are time-independent, a small subset is chosen in a time-dependent manner to adapt to the evolution of the wavepacket in phase space. We demonstrate the accuracy and efficiency of the present propagation method by calculating the electronic wavepacket in a one-dimensional soft-core atom interacting with a superposition of an intense, few-cycle, near-infrared laser pulse and an attosecond extreme-ultraviolet laser pulse.

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Norio Takemoto, Asaf Shimshovitz, David J. Tannor. 2012-05-20. Phase Space Approach to Laser-driven Electronic Wavepacket Propagation. https://doi.org/10.1063/1.4732306

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