Influence of Mg, Ag and Al substitutions on the magnetic excitations in the triangular-lattice antiferromagnet CuCrO2

Abstract

Magnetic excitations in CuCrO$_{2}$, CuCr$_{0.97}$Mg$_{0.03}$O$_{2}$, Cu$_{0.85}$Ag$_{0.15}$CrO$_{2}$, and CuCr$_{0.85}$Al$_{0.15}$O$_{2}$ have been studied by powder inelastic neutron scattering to elucidate the element substitution effects on the spin dynamics in the Heisenberg triangular-lattice antiferromagnet CuCrO$_{2}$. The magnetic excitations in CuCr$_{0.97}$Mg$_{0.03}$O$_{2}$ consist of a dispersive component and a flat component. Though this feature is apparently similar to CuCrO$_{2}$, the energy structure of the excitation spectrum shows some difference from that in CuCrO$_{2}$. On the other hand, in Cu$_{0.85}$Ag$_{0.15}$CrO$_{2}$ and CuCr$_{0.85}$Al$_{0.15}$O$_{2}$ the flat components are much reduced, the low-energy parts of the excitation spectra become intense, and additional low-energy diffusive spin fluctuations are induced. We argued the origins of these changes in the magnetic excitations are ascribed to effects of the doped holes or change of the dimensionality in the magnetic correlations.