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arXiv · 1401.4481

Failure of Logarithmic Oscillators to Thermostat Small Atomic Clusters

Daniel Sponseller·Estela Blaisten-Barojas
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Abstract

A logarithmic oscillator has the outstanding property that the expectation value of its kinetic energy is constant for all stationary states [1]. Recently the ansatz that this property can be used to define a Hamiltonian thermostat has been put forward [2]. The latter publication suggests that the logarithmic oscillator weakly coupled to a small system would serve as a thermostat as long as few degrees of freedom are involved such as in atomic clusters. We have applied these ideas to a cluster of four Lennard-Jones atoms and inspected two different models of coupling between the cluster and the logarithmic oscillator in 3D. In both cases we show that there is a clear generation of kinetic motion of the cluster center of mass, but that kinetic energy due to interatomic vibrations are not significantly affected by coupling to the logarithmic oscillator. This is a failure of the published ansatz [2], as the logarithmic oscillator is unable to modify the kinetic energy due to vibrations in small atomic clusters.

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Daniel Sponseller, Estela Blaisten-Barojas. 2014-01-17. Failure of Logarithmic Oscillators to Thermostat Small Atomic Clusters. https://doi.org/10.1103/physreve.89.021301

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