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arXiv · 1408.1978

Tm$^{3+}$:Y$_3$Ga$_5$O$_{12}$ materials for spectrally multiplexed quantum memories

Charles W. Thiel·Neil Sinclair·Wolfgang Tittel·Rufus L. Cone
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Abstract

We investigate the relevant spectroscopic properties of the 795 nm $^3$H$_6$$\leftrightarrow$$^3$H$_4$ transition in 1% Tm$^{3+}$:Y$_3$Ga$_5$O$_{12}$ at temperatures as low as 1.2 K for optical quantum memories based on persistent spectral tailoring of narrow absorption features. Our measurements reveal that this transition has uniform coherence properties over a 56 GHz bandwidth, and a simple hyperfine structure split by $\pm$44 MHz/T with lifetimes of up to hours. Furthermore, we find a $^3$F$_4$ population lifetime of 64 ms -- one of the longest lifetimes observed for an electronic level in a solid --, and an exceptionally long coherence lifetime of 490 $μ$s -- the longest ever observed for optical transitions of Tm$^{3+}$ ions in a crystal. Our results suggest that this material allows realizing broadband quantum memories that enable spectrally multiplexed quantum repeaters.

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Charles W. Thiel, Neil Sinclair, Wolfgang Tittel, Rufus L. Cone. 2014-10-22. Tm$^{3+}$:Y$_3$Ga$_5$O$_{12}$ materials for spectrally multiplexed quantum memories. https://doi.org/10.1103/physrevlett.113.160501

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