From dissipative dynamics to studies of heat transfer at the nanoscale

Nazim Boudjada; Dvira Segal

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arXiv · 1409.3201

From dissipative dynamics to studies of heat transfer at the nanoscale

Nazim Boudjada·Dvira Segal

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Abstract

We study in a unified manner the dissipative dynamics and the transfer of heat in the two-bath spin-boson model. We use the Bloch-Redfield (BR) formalism, valid in the very weak system-bath coupling limit, the noninteracting-blip approximation (NIBA), applicable in the non-adiabatic limit, and iterative, numerically-exact path integral tools. These methodologies were originally developed for the description of the dissipative dynamics of a quantum system, and here they are applied to explore the problem of quantum energy transport in a non-equilibrium setting. Specifically, we study the weak-to-intermediate system-bath coupling regime at high temperatures $k_BT/\hbar>ε$, with $ε$ as the characteristic frequency of the two-state system. The BR formalism and NIBA can lead to close results for the dynamics of the reduced density matrix (RDM) in a certain range of parameters. However, relatively small deviations in the RDM dynamics propagate into significant qualitative discrepancies in the transport behavior. Similarly, beyond the strict non-adiabatic limit NIBA's prediction for the heat current is qualitatively incorrect: It fails to capture the turnover behavior of the current with tunneling energy and temperature. Thus, techniques that proved meaningful for describing the RDM dynamics, to some extent even beyond their rigorous range of validity, should be used with great caution in heat transfer calculations, since qualitative-serious failures develop once parameters are mildly stretched beyond the techniques' working assumptions.

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Nazim Boudjada, Dvira Segal. 2014-09-10. From dissipative dynamics to studies of heat transfer at the nanoscale. https://arxiv.org/abs/1409.3201

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