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arXiv · 1512.08729

TaN, a molecular system for probing ${\cal{P,T}}$-violating hadron physics

Timo Fleig·Malaya K. Nayak·Mikhail Kozlov
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Abstract

All-electron configuration interaction theory in the framework of the Dirac-Coulomb Hamiltonian has been applied to the TaN molecule, a promising candidate in the search for Beyond-Standard-Model physics in both the hadron and the lepton sector of matter. We obtain in the first excited {$^3Δ_1$} state a ${\cal{P,T}}$-odd effective electric field of $36.0 \left[\frac{\rm GV}{\rm cm}\right]$, a scalar-pseudoscalar ${\cal{P,T}}$-odd interaction constant of $32.8$ [kHz], and a nuclear magnetic-quadrupole moment interaction constant of $0.74$ [$\frac{10^{33} {\text{Hz}}}{e\, {\text{cm}}^2}$]. The latter interaction constant has been obtained with a new approach which we describe in detail. Using the same highly correlated all-electron wavefunctions with up to $2.5$ billion expansion terms, we obtain a parallel magnetic hyperfine interaction constant of $-2954$ [MHz] for the $\rm {^{181}{T}a}$ nucleus, a very large molecule-frame electric dipole moment of $-4.91$ [Debye], and spectroscopic constants for the four lowest-lying electronic states of the molecule.

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Timo Fleig, Malaya K. Nayak, Mikhail Kozlov. 2015-11-01. TaN, a molecular system for probing ${\cal{P,T}}$-violating hadron physics. https://doi.org/10.1103/physreva.93.012505

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