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arXiv · 1603.00777

Protecting and accelerating adiabatic passage with time-delayed pulse sequences

Pablo Sampedro·Bo Y. Chang·Ignacio R. Sola
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Abstract

Using numerical simulations of two-photon electronic absorption with femtosecond pulses in Na$_2$ we show that: i) it is possible to avoid the characteristic saturation or dumped Rabi oscillations in the yield of absorption by time-delaying the laser pulses; ii) it is possible to accelerate the onset of adiabatic passage by using the vibrational coherence starting in a wave packet; and iii) it is possible to prepare the initial wave packet in order to achieve full state-selective transitions with broadband pulses. The findings can be used, for instance, to achieve ultrafast adiabatic passage by light-induced potentials and understand its intrinsic robustness.

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Pablo Sampedro, Bo Y. Chang, Ignacio R. Sola. 2016-03-02. Protecting and accelerating adiabatic passage with time-delayed pulse sequences. https://doi.org/10.1039/c6cp01680d

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