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arXiv · 1604.00814

Spin freezing in the disordered pyrochlore magnet NaCaCo$_2$F$_7$: NMR studies and Monte-Carlo simulations

R. Sarkar·J. W. Krizan·F. Brückner·E. C. Andrade·S. Rachel·M. Vojta·R. J. Cava·H. -H. Klauss
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Abstract

We present results of $^{23}$Na and $^{19}$F nuclear magnetic resonance (NMR) measurements on NaCaCo$_2$F$_7$, a frustrated pyrochlore magnet with a Curie-Weiss temperature, $T_{cw}$ ~-140 K, and intrinsic bond disorder. Below 3.6 K both the $^{23}$Na and $^{19}$F spectra broaden substantially in comparison to higher temperatures accompanied by a considerable reduction (80 \%) of the NMR signal intensity: This proves a broad quasi-static field distribution. The $^{19}$F spin-lattice relaxation rate $^{19}(1/T_1$) exhibits a peak at 2.9 K already starting to develop below 10 K. We attribute the spin freezing to the presence of bond disorder. This is corroborated by large-scale Monte-Carlo simulations of a classical bond-disordered XY model on the pyrochlore lattice. The low freezing temperature, together with the very short magnetic correlation length not captured by the simulations, suggesting that quantum effects play a decisive role in NaCaCo$_2$F$_7$.

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R. Sarkar, J. W. Krizan, F. Brückner, E. C. Andrade, S. Rachel, M. Vojta, R. J. Cava, H. -H. Klauss. 2016-04-04. Spin freezing in the disordered pyrochlore magnet NaCaCo$_2$F$_7$: NMR studies and Monte-Carlo simulations. https://doi.org/10.1103/physrevb.96.235117

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