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arXiv · 1606.08200

Molecular echoes in space and time

Kang Lin·Peifen Lu·Junyang Ma·Xiaochun Gong·Qiying Song·Qinying Ji·Wenbin Zhang·Heping Zeng·Jian Wu·Gabriel Karras·Guillaume Siour·Jean-Michel Hartmann·Olivier Faucher·Erez Gershnabel·Yehiam Prior·Ilya Sh. Averbukh
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Abstract

Mountain echoes are a well-known phenomenon, where an impulse excitation is mirrored by the rocks to generate a replica of the original stimulus, often with reverberating recurrences. For spin echoes in magnetic resonance and photon echoes in atomic and molecular systems the role of the mirror is played by a second, time delayed pulse which is able to reverse the ow of time and recreate the original event. Recently, laser-induced rotational alignment and orientation echoes were introduced for molecular gases, and discussed in terms of rotational-phase-space filamentation. Here we present, for the first time, a direct spatiotemporal analysis of various molecular alignment echoes by means of coincidence Coulomb explosion imaging. We observe hitherto unreported spatially rotated echoes, that depend on the polarization direction of the pump pulses, and find surprising imaginary echoes at negative times.

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Kang Lin, Peifen Lu, Junyang Ma, Xiaochun Gong, Qiying Song, Qinying Ji, Wenbin Zhang, Heping Zeng, Jian Wu, Gabriel Karras, Guillaume Siour, Jean-Michel Hartmann, Olivier Faucher, Erez Gershnabel, Yehiam Prior, Ilya Sh. Averbukh. 2016-06-27. Molecular echoes in space and time. https://arxiv.org/abs/1606.08200

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