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arXiv · 1609.06105

Magnetic anisotropy and the phase diagram of chiral MnSb2O6

Abstract

The magnetic phase diagram and low-energy magnon excitations of structurally and magnetically chiral MnSb2O6 are reported. The specific heat and the static magnetization are investigated in magnetic fields up to 9 and 30 T, respectively, while the dynamicmagnetic properties are probed by X-band as well as tunable high-frequency electron spin-resonance spectroscopy. Below TN = 11.5 K, we observe antiferromagnetic resonance modes which imply small but finite planar anisotropy showing up in a zero-field splitting of 20 GHz. The data are well described by means of an easy-plane two-sublattice model with the anisotropy field BA = 0.02 T. The exchange field BE = 13 T is obtained from the saturation field derived from the pulsed-field magnetization. A crucial role of the small anisotropy for the spin structure is reflected by competing antiferromagnetic phases appearing, at T = 2 K, in small magnetic fields at BC1 $\approx$ 0.5 T and BC2 = 0.9 T. We discuss the results in terms of spin reorientation and of small magnetic fields favoring helical spin structure over the cycloidal ground state which, at B = 0, is stabilized by the planar anisotropy. Above TN, short-range magnetic correlations up to >=60 K and magnetic entropy changes well above TN reflect the frustrated triangular arrangement of Mn2+ ions in MnSb2O6.

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BibTeXRIS

J. Werner, C. Koo, R. Klingeler, A. N. Vasiliev, Y. A. Ovchenkov, A. S. Polovkova, G. V. Raganyan, E. A. Zvereva. 2016-09-20. Magnetic anisotropy and the phase diagram of chiral MnSb2O6. https://doi.org/10.1103/physrevb.94.104408

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