Search arXivSearch

arXiv · 1612.03987

Morphology of clusters of attractive dry and wet self-propelled spherical particle suspensions

Abstract

In order to asses the effect of hydrodynamics in the assembly of active attractive spheres, we simulate a semi-dilute suspension of attractive self-propelled spherical particles in a quasi two dimensional geometry comparing the case with and without hydrodynamics interactions. To start with, independently on the presence of hydrodynamics, we observe that depending on the ratio between attraction and propulsion, particles either coarsen or aggregate forming finite-size clusters. Focusing on the clustering regime, we characterize two different clusters parameters, i.e. their morphology and orientational order, and compare the case when active particles behave either as pushers or pullers (always in the regime where inter-particles attractions competes with self-propulsion). Studying cluster phases for squirmers with respect to those obtained for active Brownian disks (indicated as ABP), we have shown that hydrodynamics alone can sustain a cluster phase of active swimmers (pullers), while ABP form cluster phases due to the competition between attraction and self propulsion. The structural properties of the cluster phases of squirmers and ABP are similar, although squirmers show sensitivity to active stresses. Active Brownian disks resemble weakly pusher squirmer suspensions in terms of cluster size distribution, structure of the radius of gyration on cluster size and degree of cluster polarity.

Explore related subjects

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

Francisco Alarcón, Chantal Valeriani, Ignacio Pagonabarraga. 2016-12-14. Morphology of clusters of attractive dry and wet self-propelled spherical particle suspensions. https://doi.org/10.1039/c6sm01752e

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

Transient Elasticity -- A Unifying Framework for Thixotropy, Polymers, and Granular Media

Thixotropic yield stress fluids, such as paint or ketchup, are traditionally viewed as elastic structures that, under shear rates, break into viscous liquids with lumps, and reconnect at rest. An alternative framework is presented here: Upon shear, structural destruction is incomplete, leaving sufficient connections. As a result, elasticity fundamentally underlies their non-Newtonian behavior, though they do appear purely viscous under a steady shear, displaying little direct evidence of elastic rebound---same as granular media and polymers. Consequently, all three are described by the same set of evolution equations, differing only in their parameters. These equations are set up by starting from solid dynamics and allowing the elastic strain $\varepsilon^e$ to relax, which in effect interpolates between solid and fluid behavior, appropriate for systems that display both types of behavior. Incorporating in addition a two-temperature framework, tracking how energy is dissipated in two consecutive stages, yields the nonlinear model of Transient Elasticity (TE). It describes an elasticity that is transient in time yet persistent under shear. Previously validated for polymers and granular media, TE is here applied to thixotropic yield-stress fluids. As shown, it successfully accounts for a wide range of characteristic phenomena, including over- and undershoot, viscosity bifurcation, shear banding, and oscillatory rheography. Given its appropriateness across structurally diverse systems, TE offers a unified, surprisingly general account of non-Newtonian phenomena.

cond-mat.soft

Deformation and organization of droplet-encapsulated soft beads

Many biological, culinary, and engineering processes lead to the co-encapsulation of several soft particles within a liquid interface. In these situations the particles are bound together by the capillary forces that deform them and influence their biological or rheological properties. Here, we introduce an experimental approach to encapsulate a controlled number of soft beads within aqueous droplets in oil. These droplet-encapsulated gels are manipulated in a deformable microfluidic device to merge them and modify the liquid fraction. In the dry limit the contact surface between the hydrogels is found to be determined by the elastocapillary number $E_c$, with the contact radius following a $E_c^{1/3}$ dependence, indicating that the deformation increases for soft or small particles. When multiple beads are co-encapsulated within a single droplet they can be arranged into linear or three-dimensional aggregates that remain at a local energy minimum.

cond-mat.soft

Flexoelectricity-driven softening of bend elasticity leads to spontaneous chiral symmetry breaking in a polar fluid

The origin of the recently observed spontaneous chiral symmetry breaking in polar fluids composed of achiral molecules is an unsolved problem, raising fundamental questions about how heliconical structures emerge in such systems. Here, we investigate the pretransitional fluctuations leading to the formation of the spontaneously chiral twist-bend ferroelectric nematic phase using dielectric spectroscopy, light scattering, and small-angle X-ray scattering. We observe simultaneous softening of the bend elastic constant and the emergence of a collective dielectric mode on approaching the transition. By developing a theoretical model, we show that these phenomena are signatures of a flexoelectricity-driven transition arising from the coupling between electric polarization and bend deformation.

cond-mat.soft