Search arXivSearch

arXiv · 1704.08850

BCS-like critical fluctuations with limited overlap of Cooper pairs in FeSe

Abstract

In conventional superconductors, very narrow superconducting fluctuation regions are observed above $T_c$ because of the strong overlapping of Cooper pairs in a coherence volume. In the bulk form of iron chalcogenide superconductor FeSe, it is argued that the system may locate in the crossover region of BCS to BEC, indicating a strong superconducting fluctuation. In this respect, we have carried out measurements of magnetization, specific heat and Nernst effect on FeSe single crystals in order to investigate the superconducting fluctuation effect near $T_c$. The region of diamagnetization induced by superconducting fluctuation seems very narrow above $T_c$. The crossing point of temperature dependent magnetization curves measured at different magnetic fields, which appears in many systems of cuprate superconductors and is regarded as indication of strong critical fluctuation, is however absent. The magnetization data can be scaled based on the Ginzburg-Landau fluctuation theory for a quasi-two-dimensional system, but the scaling result cannot be described by the theoretical function of the fluctuation theory because of the limited fluctuation regions. The specific heat jump near $T_c$ is rather sharp without the trace of strong superconducting fluctuation. This is also supported by the Nernst effect measurements which indicate a very limited region for vortex motion above $T_c$. Associated with very small value of Ginzburg number and further analyses, we conclude that the superconducting fluctuation is very weak above $T_c$ in this material. Our results are strongly against the picture of significant phase fluctuation in FeSe single crystals, although the system has a very limited overlapping of Cooper pairs in the coherence volume. This dichotomy provides new insights into the superconducting mechanism when the system is with a dilute superfluid density.

Explore related subjects

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

Huan Yang, Guanyu Chen, Xiyu Zhu, Jie Xing, Hai-Hu Wen. 2017-07-14. BCS-like critical fluctuations with limited overlap of Cooper pairs in FeSe. https://doi.org/10.1103/physrevb.96.064501

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

Superconductivity in MgHCu3 perovskite revisited

We reexamine the crystal structure, electronic structure, lattice dynamics, phonon dispersion, electron-phonon coupling, and superconducting properties of MgHCu3 perovskite using the PBEsol and PBE functionals. This perovskite phase was recently proposed to exhibit superconductivity with the critical superconducting temperature, TC, of 42 K, which falls slightly over the classical 40 K limit for the phonon driven superconductivity. We show that although the crystal and electronic structure of this hypothetical compound are quite robust with respect to the k point mesh and functional used, yet the phonons and phonon related properties are extremely sensitive to the density of the grid chosen as well as functional used for calculations. Correspondingly, the values of the critical superconducting temperature calculated here for different Gaussian broadenings vary in a broad range of ca. 10 to 31 K and they do not exceed the classical limit. We suggest that the properties of this and many other high TC hydrides claimed should be thoroughly scrutinized using a variety of functionals, and benchmarked with experiment, to provide more reliable values of TC.

cond-mat.supr-con

Multigap superconductivity in Ising superconductors: The case of (LaSe)1.14(NbSe2)m misfit layer compounds

Strong spin-orbit coupling and broken inversion symmetry in transition metal dichalcogenides give rise to Ising superconductivity, a spin-protected pairing state first identified in monolayer NbSe$_2$ through in-plane critical fields far exceeding the Pauli limit. More recently, Ising superconductivity has been proposed as a potential route to unconventional and even topological superconductivity in bulk misfit compounds. Here, we investigate the superconducting order parameter of layered misfit compounds composed of alternating transition metal dichalcogenide and rocksalt layers, which host extremely doped, electronically decoupled NbSe$_2$ sheets within a three-dimensional crystal. Using directional scanning tunneling spectroscopy on the misfit superconductors (LaSe)$_{1.14}$(NbSe$_2$) and (LaSe)$_{1.14}$(NbSe$_2$)$_2$, we uncover a strongly anisotropic multigap superconducting state: a fragile gap on the $Γ$-centered Fermi-surface pocket coexists with a robust, intrinsic gap on the K and K$'$ pockets. These features are in quantitative agreement with momentum-resolved gaps $Δ(\mathbf{k})$ obtained from anisotropic Migdal-Eliashberg calculations. The marked fragility of the $Γ$-centered gap, combined with the strong sensitivity of the critical temperature to non-magnetic disorder, points to pairing beyond conventional $s$-wave symmetry, potentially involving a topological order parameter. These results establish NbSe$_2$-based misfit compounds as a tunable bulk platform for multigap, unconventional superconductivity, with Ising protection offering a promising route toward topological pairing.

cond-mat.supr-con

Different reconstruction pathways toward superconductivity in TaRhTe4 and TaIrTe4 Weyl semimetals

Pressure can drive Weyl semimetals toward superconductivity through qualitatively distinct reconstructions of their lattices and normal-state electronic structures. Here, we report the first observation of superconductivity in compressed TaRhTe4. This finding enables a direct comparison of the distinct reconstruction pathways leading to superconductivity in TaRhTe4 and the previously studied TaIrTe4, both of which belong to the TaXTe4 (X = Rh, Ir) family of type-II Weyl semimetals. For TaRhTe4, high-pressure electrical-resistance, Hall effect, and magnetoresistance measurements, together with synchrotron X-ray diffraction and first-principles calculations, reveal a superconducting transition that emerges near 20 GPa, with onset Tc increasing to approximately 2.6 K at 65.2 GPa and zero resistance achieved above 63 GPa. The onset of superconductivity coincides with a progressive lattice distortion, a strong suppression of the positive magnetoresistance, and a continuous decrease of the Hall coefficient toward zero. Calculations further show that additional electron-like bands cross the Fermi level (EF) and that N(EF) increases upon compression. This evolution contrasts with TaIrTe4, where the Hall coefficient initially increases before reversing its pressure dependence near the superconducting threshold, while the structural anomaly is confined to a narrower pressure interval. This comparison indicates that superconductivity in the TaXTe4 family is not tied to a unique critical pressure or a single Fermi-surface reconstruction, but can emerge through distinct material-specific pathways once pressure sufficiently reconstructs the low-carrier Weyl-semimetal-derived state into a multiband metallic regime.

cond-mat.supr-con