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arXiv · 1806.05014

Harmonic Generation from Metal-Oxide and Metal-Metal Boundaries

M. Scalora·M. A. Vincenti·D. de Ceglia·N. Akozbek·M. J. Bloemer·C. De Angelis·J. W. Haus·R. Vilaseca·J. Trull·C. Cojocaru
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Abstract

We explore the outcomes of detailed microscopic models by calculating second- and third-harmonic generation from thin film surfaces with discontinuous free-electron densities. These circumstances can occur in structures consisting of a simple metal mirror, or arrangements composed of either different metals or a metal and a free electron system like a conducting oxide. Using a hydrodynamic approach we highlight the case of a gold mirror, and that of a two-layer system containing indium tin oxide (ITO) and gold. We assume the gold mirror surface is characterized by a free-electron cloud of varying density that spills into the vacuum, which as a result of material dispersion exhibits epsilon-near-zero conditions and local field enhancement at the surface. For a bylayer consisting of a thin ITO and gold films, if the wave is incident from the ITO side the electromagnetic field is presented with a free-electron discontinuity at the ITO/gold interface, and wavelength-dependent, epsilon-near-zero conditions that enhance local fields and conversion efficiencies, and determine the surface's emission properties. We evaluate the relative significance of additional nonlinear sources that arise when a free-electron discontinuity is present, and show that harmonic generation can be sensitive to the density of the screening free-electron cloud, and not its thickness. Our findings also suggest the possibility to control surface harmonic generation through surface charge engineering.

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M. Scalora, M. A. Vincenti, D. de Ceglia, N. Akozbek, M. J. Bloemer, C. De Angelis, J. W. Haus, R. Vilaseca, J. Trull, C. Cojocaru. 2018-06-13. Harmonic Generation from Metal-Oxide and Metal-Metal Boundaries. https://doi.org/10.1103/physreva.98.023837

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