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arXiv · 1905.11186

Spin relaxation in Cs$_2$CuCl$_{4-x}$Br$_x$

R. Hassan Abadi·R. M. Eremina·M. Hemmida·A. Dittl·B. Wolf·W. Assmus·A. Loidl·H. -A. Krug von Nidda
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Abstract

The quantum-spin S = 1=2 chain system Cs$_2$CuCl$_4$ is of high interest due to competing anti-ferromagnetic intra-chain J and inter-chain exchange J' interactions and represents a paramount example for Bose-Einstein condensation of magnons [R. Coldea et al., Phys. Rev. Lett. 88, 137202 (2002)]. Substitution of chlorine by bromine allows tuning the competing exchange interactions and corresponding magnetic frustration. Here we report on electron spin resonance (ESR) in single crystals of Cs$_2$CuCl$_{4-x}$Br$_x$ with the aim to analyze the evolution of anisotropic exchange contributions. The main source of the ESR linewidth is attributed to the uniform Dzyaloshinskii-Moriya interaction. The vector components of the Dzyaloshinskii-Moriya interaction are determined from the angular dependence of the ESR spectra using a high-temperature approximation. The obtained results support the site selectivity of the Br substitution suggested from the evolution of lattice parameters and magnetic susceptibility dependent on the Br concentration.

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R. Hassan Abadi, R. M. Eremina, M. Hemmida, A. Dittl, B. Wolf, W. Assmus, A. Loidl, H. -A. Krug von Nidda. 2019-05-27. Spin relaxation in Cs$_2$CuCl$_{4-x}$Br$_x$. https://doi.org/10.1103/physrevb.103.064420

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