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arXiv · 1906.10763

Magnetic Ordering in the Ising Antiferromagnetic Pyrochlore Nd2ScNbO7

Cole Mauws·Nathaniel Hiebert·Megan Rutherford·Haidong D. Zhou·Qing Huang·Matthew B. Stone·Nicholas P. Butch·Yixi Su·Eun Sang Choi·Zahra Yamani·Christopher R. Wiebe
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Abstract

The question of structural disorder and its effects on magnetism is relevant to a number of spin liquid candidate materials. Although commonly thought of as a route to spin glass behavior, here we describe a system in which the structural disorder results in long-range antiferromagnetic order due to local symmetry breaking. Nd$_2$ScNbO$_7$ is shown to have a dispersionless gapped excitation observed in other neodymium pyrochlores below T$_N$ = 0.37 K through polarized and inelastic neutron scattering. However the dispersing spin waves are not observed. This excited mode is shown to occur in only 14(2) \% of the neodymium ions through spectroscopy and is consistent with total scattering measurements as well as the magnitude of the dynamic moment 0.26(2) $μ_B$. The remaining magnetic species order completely into the all-in all-out Ising antiferromagnetic structure. This can be seen as a result of local symmetry breaking due disordered Sc$^{+3}$ and Nb$^{+5}$ ions about the A-site. From this work, it has been established that B-site disorder restores the dipole-like behaviour of the Nd$^{+3}$ ions compared to the Nd$_2$B$_2$O$_7$ parent series.

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Cole Mauws, Nathaniel Hiebert, Megan Rutherford, Haidong D. Zhou, Qing Huang, Matthew B. Stone, Nicholas P. Butch, Yixi Su, Eun Sang Choi, Zahra Yamani, Christopher R. Wiebe. 2021-03-31. Magnetic Ordering in the Ising Antiferromagnetic Pyrochlore Nd2ScNbO7. https://arxiv.org/abs/1906.10763

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