Search arXivSearch

arXiv · 1912.02603

Iron-based superconductors: tales from the nuclei

Abstract

High-temperature superconductivity in Fe-based pnictides and chalcogenides has been one of the most significant recent discoveries in condensed matter physics and has attracted remarkable attention in the last decade. These materials are characterized by a complex fermiology and, as a result, feature a wide range of electronic properties as a function of different tuning parameters such as chemical doping, temperature and pressure. Along the path towards the comprehension of the physical mechanisms underlying this rich phenomenology, NMR (nuclear magnetic resonance) and NQR (nuclear quadrupole resonance) have played a role of capital importance that we review in this work. In particular, we address how NMR has contributed to the current understanding of the main regions of the electronic phase diagram of Fe-based pnictides, that is, the -- sometimes coexisting -- antiferromagnetic spin-density wave and superconducting states. We evidence the unique capability of NMR as local-probe technique of investigating the effect of quenched disorder and chemical impurities. Then, we review the NMR signatures of low-frequency fluctuations associated with the development of electronic nematicity as well as with the motion of superconducting flux lines. Finally, we discuss recent contributions of NMR and NQR which evidence an intrinsically inhomogeneous electronic charge distribution as well as an orbitally-selective behaviour.

Explore related subjects

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

Pietro Carretta, Giacomo Prando. 2019-12-05. Iron-based superconductors: tales from the nuclei. https://doi.org/10.1007/s40766-019-0001-1

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

Superconductivity in MgHCu3 perovskite revisited

We reexamine the crystal structure, electronic structure, lattice dynamics, phonon dispersion, electron-phonon coupling, and superconducting properties of MgHCu3 perovskite using the PBEsol and PBE functionals. This perovskite phase was recently proposed to exhibit superconductivity with the critical superconducting temperature, TC, of 42 K, which falls slightly over the classical 40 K limit for the phonon driven superconductivity. We show that although the crystal and electronic structure of this hypothetical compound are quite robust with respect to the k point mesh and functional used, yet the phonons and phonon related properties are extremely sensitive to the density of the grid chosen as well as functional used for calculations. Correspondingly, the values of the critical superconducting temperature calculated here for different Gaussian broadenings vary in a broad range of ca. 10 to 31 K and they do not exceed the classical limit. We suggest that the properties of this and many other high TC hydrides claimed should be thoroughly scrutinized using a variety of functionals, and benchmarked with experiment, to provide more reliable values of TC.

cond-mat.supr-con

Different reconstruction pathways toward superconductivity in TaRhTe4 and TaIrTe4 Weyl semimetals

Pressure can drive Weyl semimetals toward superconductivity through qualitatively distinct reconstructions of their lattices and normal-state electronic structures. Here, we report the first observation of superconductivity in compressed TaRhTe4. This finding enables a direct comparison of the distinct reconstruction pathways leading to superconductivity in TaRhTe4 and the previously studied TaIrTe4, both of which belong to the TaXTe4 (X = Rh, Ir) family of type-II Weyl semimetals. For TaRhTe4, high-pressure electrical-resistance, Hall effect, and magnetoresistance measurements, together with synchrotron X-ray diffraction and first-principles calculations, reveal a superconducting transition that emerges near 20 GPa, with onset Tc increasing to approximately 2.6 K at 65.2 GPa and zero resistance achieved above 63 GPa. The onset of superconductivity coincides with a progressive lattice distortion, a strong suppression of the positive magnetoresistance, and a continuous decrease of the Hall coefficient toward zero. Calculations further show that additional electron-like bands cross the Fermi level (EF) and that N(EF) increases upon compression. This evolution contrasts with TaIrTe4, where the Hall coefficient initially increases before reversing its pressure dependence near the superconducting threshold, while the structural anomaly is confined to a narrower pressure interval. This comparison indicates that superconductivity in the TaXTe4 family is not tied to a unique critical pressure or a single Fermi-surface reconstruction, but can emerge through distinct material-specific pathways once pressure sufficiently reconstructs the low-carrier Weyl-semimetal-derived state into a multiband metallic regime.

cond-mat.supr-con

Electromagnetic Proximity Effects and Spontaneous Currents in Clean Superconducting Heterostructures

When ferromagnets are brought into contact with a superconductor, superconducting proximity effects give rise to a variety of interesting phenomena, including oscillatory singlet Cooper-pair amplitudes and long-ranged odd-frequency triplet correlations induced by the exchange interactions in the ferromagnets. From an electrodynamic perspective, however, it is equally important to understand when and how spontaneous currents can emerge. To investigate the interplay between electromagnetic and conventional superconducting proximity effects, we study clean ferromagnet/ferromagnet/superconductor spin-valve heterostructures in which the relative angle between the two ferromagnetic layers can be tuned. Our approach is based on a self-consistent numerical solution of the coupled Bogoliubov-de Gennes and Maxwell equations, providing a microscopic description capable of resolving physics on atomic length scales. Several notable features emerge. In both the weak- and strong-exchange-field regimes, the central ferromagnetic layer plays a dominant role in generating sizable spontaneous currents when its exchange-field strength is varied. We further find that the resulting electromagnetic response extends across the entire superconducting layer, in sharp contrast to the short-ranged inverse proximity effect. In noncollinear configurations, the electromagnetic proximity effect also reconfigures the local magnetic-field orientation and reduces the angular mismatch between the fields in the two ferromagnetic layers. The long-ranged odd-frequency triplet amplitudes are consequently modified by the orbital response, which alters the underlying quasiparticle states by changing their momentum-space structure. Finally, our framework can be naturally generalized to other superconducting spintronic systems, possibly including Josephson junctions and altermagnet/superconductor heterostructures.

cond-mat.supr-con