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arXiv · 2008.12012

Microscopic evidence for the intra-unit-cell electronic nematicity inside the pseudogap phase in YBa$_2$Cu$_4$O$_8$

W. Wang·J. Luo·C. G. Wang·J. Yang·Y. Kodama·R. Zhou·Guo-qing Zheng
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Abstract

Understanding the nature of the mysterious pseudogap phenomenon is one of the most important issues associated with cuprate high-$T_c$ superconductors. Here, we report $^{17}$O nuclear magnetic resonance (NMR) studies on two planar oxygen sites in stoichiometric cuprate YBa$_2$Cu$_4$O$_8$ to investigate the symmetry breaking inside the pseudogap phase. We observe that the Knight shifts of the two oxygen sites are identical at high temperatures but different below $T_{\rm nem} \sim$ 185 K, which is close to the pseudogap temperature $T^{\ast}$. Our result provides a microscopic evidence for intra-unit-cell electronic nematicity. The difference in quadrupole resonance frequency between the two oxygen sites is unchanged below $T_{\rm nem}$, which suggests that the observed nematicity does not directly stem from the local charge density modulation. Furthermore, a short-range charge density wave (CDW) order is observed below $T \simeq$ 150 K. The additional broadening in the $^{17}$O-NMR spectra because of this CDW order is determined to be inequivalent for the two oxygen sites, which is similar to that observed in case of nematicity. These results suggest a possible connection between nematicity, CDW order, and pseudogap.

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W. Wang, J. Luo, C. G. Wang, J. Yang, Y. Kodama, R. Zhou, Guo-qing Zheng. 2020-08-27. Microscopic evidence for the intra-unit-cell electronic nematicity inside the pseudogap phase in YBa$_2$Cu$_4$O$_8$. https://doi.org/10.1007/s11433-020-1615-y

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