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arXiv · 2105.06875

Chiral Order and Multiferroic Domain Relaxation in NaFeGe$_2$O$_6$

S. Biesenkamp·D. Gorkov·W. Schmidt·K. Schmalzl·Y. Sidis·P. Becker·L. Bohatý·M. Braden
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Abstract

The magnetic structure and the multiferroic relaxation dynamics of NaFeGe$_2$O$_6$ were studied by neutron scattering on single crystals partially utilizing polarization analysis. In addition to the previously reported transitions, the incommensurate spiral ordering of Fe$^{3+}$ moments in the $ac$ plane develops an additional component along the crystallographic $b$ direction below $T\approx 5\text{ K}$, which coincides with a lock-in of the incommensurate modulation. The quasistatic control of the spin-spiral handedness, respectively of the vector chirality, by external electric fields proves the invertibility of multiferroic domains down to the lowest temperature. Time-resolved measurements of the multiferroic domain inversion in NaFeGe$_2$O$_6$ reveal a simple temperature and electric-field dependence of the multiferroic relaxation that is well described by a combined Arrhenius-Merz relation, as it has been observed for TbMnO$_3$. The maximum speed of domain wall motion is comparable to the spin wave velocity.

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S. Biesenkamp, D. Gorkov, W. Schmidt, K. Schmalzl, Y. Sidis, P. Becker, L. Bohatý, M. Braden. 2021-05-14. Chiral Order and Multiferroic Domain Relaxation in NaFeGe$_2$O$_6$. https://doi.org/10.1103/physrevb.104.174405

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