Search arXivSearch

arXiv · 2108.08335

Exploring an experimental route of synthesizing superheavy elements beyond Z > 118

Abstract

Role of the Coulomb interaction, mean fissility, mass asymmetry, and charge asymmetry parameters on the synthesis of heavy and superheavy elements has been examined with respect to the deformation parameters of the projectile and target nuclei explicitly in light of the experimental results. The observed facts are classified into four categories and are then used to study several unsuccessful as well as planned reactions to synthesize the new superheavy elements $Z= 119, 120$. Concrete inference is too difficult to draw from these results because of excessive deviations in evaporation residue cross-section data. It is found that the arbitrary choice of excitation energy for the experiments studied was the root cause of such large deviations. Such a complex issue can be resolved well by theoretical excitation function studies using the advanced statistical model or the dinuclear system model and choosing the excitation energy corresponding to the energy where the excitation function curve shows the maximum. We believe this method may help us to predict whether the estimated evaporation residue cross-section can be measurable within the experimental limit of the existing facilities for the future reactions planned.

Explore related subjects

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

H. C. Manjunatha, Y. S. Vidya, P. S. Damodara Gupta, N. Manjunatha, N. Sowmya, L. Seenappa, T. Nandi. 2021-08-18. Exploring an experimental route of synthesizing superheavy elements beyond Z > 118. https://arxiv.org/abs/2108.08335

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

Three-dimensional orbital-free density functional theory description of nuclear pasta in the inner crust of neutron stars

Background: In the bottom layer of the inner crust of neutron stars, various crystalline structures are expected to emerge that are collectively called ``nuclear pasta.'' It is desirable to know properties of nuclear pasta in a wide variety of conditions for astrophysical applications. However, three-dimensional fully-microscopic calculations require huge computational effort that makes it still challenging to carry out systematic calculations. Purpose: In this paper, we propose an efficient method to calculate various nuclear pasta configurations in a non-empirical manner, based on three-dimensional orbital-free density functional theory (OF-DFT). We demonstrate the feasibility of the proposed approach by applying it to densities across the inner crust of neutron stars. Methods: As a first application of OF-DFT for nuclear pasta, we employ the second-order extended Thomas-Fermi (ETF) expansion of Skyrme energy density functional (EDF) to construct an EDF that depends only on neutron and proton number densities. Based on the variational principle, we derive Euler-Lagrange equations to determine optimal neutron and proton density distributions and solve them self-consistently. In this work, we call this approach the self-consistent ETF (SC-ETF) method. Results: We perform three-dimensional SC-ETF calculations with various box sizes. We successfully obtain various pasta structures, depending on given average nucleon number densities, consistent with earlier studies. Moreover, we find other exotic structures, such as bending and/or connected rods, slabs with a hole, etc., underlining the advantage of the self-consistent formalism. Conclusions: We demonstrate that the SC-ETF method proposed in this study, which can be regarded as a realization of OF-DFT, is a promising tool that can efficiently describe complex pasta structures without empirical assumptions on geometric shapes.

nucl-th

Microscopic analysis of M1 scissors mode in $^{254}$No

The low-energy $M1$ orbital scissors mode (SM) was recently observed by Oslo group in deformed nucleus $^{254}$No. This is the heaviest nucleus where SM was ever experimentally found. We propose the analysis of SM, together with the spin-flip $M1$ resonance, within fully self-consistent Quasiparticle Random-Phase Approximation (QRPA) with Skyrme forces SG2, SLy4 and SLy5. The impact of "tensor" $J^2$-term, introduced by perturbative (on the base of SG2) and consistent (SLy5) ways, is analyzed and shown to be noticeable but not decisive. The deformation-induced coupling of $M1$ and $E2$ states is inspected. The calculations reasonably describe Oslo's experimental data. The best agreement is obtained for SLy5. A fine structure of SM in $^{254}$No is predicted. A significant constructive interference of the dominant orbital and minor spin-flip contributions to $M1$ strength at SM energy region is found. What is remarkable, our analysis of distributions of the convective nuclear currents challenges the scissors-like flow usually assumed for SM.

nucl-th

Systematic Study of Proton, Two-Proton, Alpha, and Cluster Radioactivity Half-Lives based on the Deformed Gamow-like Model and Tabular Prior-data Fitted Network ($\mathrm{TabPFN}$)

A hybrid framework combining the deformed Gamow-like model ($\mathrm{DGLM}$) with the Tabular Prior-data Fitted Network ($\mathrm{TabPFN}$) is developed to improve half-life predictions for two-proton emission, proton emission, $α$ decay, and cluster radioactivity. A total of 583 radioactive nuclei are investigated, including 17 two-proton emitters, 42 proton emitters, 498 $α$ emitters, and 26 cluster emitters. Among the four considered models, $\mathrm{DGLM}^{b}+\mathrm{TabPFN}$ achieves the best overall performance, with $σ_{\mathrm{RMS}}=0.423$, corresponding to an improvement of approximately $82.2\%$ over $\mathrm{DGLM}^{b}$. The model parameters are optimized for each decay mode using the least-squares method. After introducing $\mathrm{TabPFN}$, the prediction errors for proton emission and $α$ decay are reduced by approximately $80.6\%$ and $87.6\%$, respectively. For $α$ decay, the training, test, and overall RMSEs are 0.208, 0.305, and 0.240, indicating good generalization capability without evident overfitting. The model also reproduces the systematic evolution of $α$-decay half-lives and the shell-closure effect around $N=126$. These results demonstrate that combining $\mathrm{DGLM}$ with $\mathrm{TabPFN}$ significantly improves the accuracy and robustness of radioactive-decay half-life predictions while retaining the physical interpretability of the original model.

nucl-th