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arXiv · 2201.11243

Slow spin dynamics in the hyper-honeycomb Lattice [(C2H5)3NH]2Cu2(C2O4)3 revealed by 1H NMR studies

Q. -P. Ding·C. Dissanayake·Santanu Pakhira·W. J. Newsome·F. Uribe-Romo·D. C. Johnston·Y. Nakajima·Y. Furukawa
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Abstract

We report the results of magnetic susceptibility $χ$ and $^1$H nuclear magnetic resonance (NMR) measurements on a three-dimensional hyper-honeycomb lattice compound [(C$_2$H$_5$)$_3$NH]$_2$Cu$_2$(C$_2$O$_4$)$_3$ (CCCO). The average value of the antiferromagnetic (AFM) exchange coupling between the Cu$^{2+}$ ($S$ = 1/2) spins was determined to be $J$~$\sim$~50 K from the $χ$ measurements. No long-range magnetic ordering has been observed down to $T$ = 50 mK, although NMR lines become slightly broader at low temperatures below 1 K. The broadening of the NMR spectrum observed below 1 K reveals that the Cu spin moments remain at this temperature, suggesting a non-spin-singlet ground state. The temperature and magnetic field dependence of 1/$T_1$ at temperatures above 20 K is well explained by paramagnetic thermal spin fluctuations where the fluctuation frequency of Cu$^{2+}$ spins is higher than the NMR frequency of the order of MHz. However, a clear signature of the slowing down of the Cu$^{2+}$ spin fluctuations was observed at low temperatures where 1/$T_1$ shows a thermally-activated behavior. The magnetic field dependence of the magnitude of the spin excitation gap suggests that the magnetic behaviors of CCCO are characterized as an AFM chain at low temperatures.

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Q. -P. Ding, C. Dissanayake, Santanu Pakhira, W. J. Newsome, F. Uribe-Romo, D. C. Johnston, Y. Nakajima, Y. Furukawa. 2022-03-02. Slow spin dynamics in the hyper-honeycomb Lattice [(C2H5)3NH]2Cu2(C2O4)3 revealed by 1H NMR studies. https://doi.org/10.1103/physrevb.105.l100405

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