Search arXiv⌕ Search
Home/Archive/arXiv

arXiv · 2212.14483

Electro-Thermo-Plasmonic Flow in Gold Nanoparticle Suspensions: Nonlinear Flow Velocity Dependence with Aggregates Concentration

Carlos David González Gómez·Raúl A. Rica·Emilio Ruiz-Reina
View original source ↗Read source document ↗Export metadata ↓

Abstract

Efficient mixing and pumping of liquids at the microscale is a technology that is still to be optimized. The combination of an AC electric field with a small temperature gradient leads to a strong electro-thermal flow that can be used for multiple purposes. Combining simulations and experiments, an analysis of the performance of electro-thermal flow is provided when the temperature gradient is generated by illuminating plasmonic nanoparticles in suspension with a near-resonance focused laser. Fluid flow is measured by tracking the velocity of fluorescent tracer microparticles in suspension as a function of the electric field, laser power, and concentration of plasmonic particles. Among other results, a non-linear relationship is found between the velocity of the fluid and particle concentration, which is justified in terms of multiple scattering-absorption events, involving aggregates and individual particles, that lead to enhanced absorption when the concentration is raised. Simulations provide a description of the phenomenon that is compatible with experiments and constitute a way to understand and estimate the absorption and scattering cross-sections of dispersed particles and/or aggregates. A comparison of experiments and simulations suggests that the gold nanoparticles are aggregated forming clusters of about 5-9 particles, but no information about their structure cannot be obtained without further theoretical and experimental developments. This nonlinear behavior could be useful to get very high ETP velocities by inducing some controlled aggregation of the particles.

Explore related subjects

physics.flu-dyncond-mat.mes-hallphysics.app-phphysics.optics

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

Carlos David González Gómez, Raúl A. Rica, Emilio Ruiz-Reina. 2022-12-29. Electro-Thermo-Plasmonic Flow in Gold Nanoparticle Suspensions: Nonlinear Flow Velocity Dependence with Aggregates Concentration. https://doi.org/10.1016/j.jcis.2023.05.198

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

arXiv2026

Mathematical modeling on peristaltic flow of a Prandtl fluid with effects of slip conditions and inclined magnetic field

The manuscript provides a description of a theoretical analysis of a non-Newtonian Prandtl fluid subject to peristaltic flow through an inclined asymmetric channel. We explore the effect of an inclined magnetic field on the peristaltic flow. This is relevant for applications involving fluid flow in narrow, inclined (tilted) tubes similar to blood vessels or the digestive system. The model also includes thermodynamic aspects such as heat diffusion (the Soret effect) and viscous dissipation resulting from wall-fluid slip conditions, which may help optimize medical devices such as lab-on-a-chip systems and dialysis machines. In this study, the concentration of a generic chemical, temperature, and fluid velocity are taken into account through mass, heat, and momentum balances, respectively. The solution is approximated using numerical techniques suitable for long wavelengths (low frequency) and low Reynolds numbers. The study also discusses trapping phenomena, which are crucial from a clinical point of view. The developed insights can improve the understanding of physiological flows in the gastrointestinal tract and blood vessels. By understanding how the fluid moves and how particles are trapped, these insights may contribute to the design of improved medical pumps and artificial organs. Graphical visualizations are provided for the fluid velocity profile, temperature distribution, and concentration of a generic chemical. Furthermore, the numerical results are validated through comparison with a closed-form solution from a benchmark problem.

physics.flu-dyn↗
arXiv2026

Discovery of a dispersion model at high Peclet numbers

Peclet number characterises the transition from classical Taylor-Aris dispersion to convection-dominated longitudinal solute transport, with the classical model becoming inadequate at extremely high radial Peclet number $Pe_r$. We develop a novel explicit-closure one-dimensional (1-D) effective dispersion model for this high-$Pe_r$ regime by introducing two closure coefficients, $θ_u$ and $θ_d$, whose functional structures are identified using low-frequency transfer-function matching and a modified Kolmogorov-Arnold network (KAN). The resulting model captures the transition from classical Taylor-Aris dispersion at low $Pe_r$ to convection-dominated dispersion at high $Pe_r$. Analysis reveals that, in the high-$Pe_r$ regime, axial transport is redistributed between the effective convection flux and the dispersive flux, resulting in a reduced macroscopic convection velocity. Numerical validation demonstrates close agreement with the convection-diffusion model over the investigated high-$Pe_r$ conditions, while the classical Taylor-Aris model exhibits substantial deviations. Application of the proposed model to averaged flow velocity inversion further demonstrates improved velocity estimation, particularly in the high-$Pe_r$ regime. These results highlight the importance of accounting for non-classical dispersion for reliable contrast-agent-based arterial blood flow velocimetry and provide new insight into high-$Pe_r$ mass transport.

physics.flu-dyn↗
arXiv2026

Optimization of fluid mixing by reinforcement learning using limit cycles of a dynamical system

We propose a method to overcome the difficulties encountered when applying reinforcement learning to fluid mixing processes. The proposed method has two main features: (i) it does not require detailed measurements of the flow state, and (ii) by effectively exploiting a stable limit cycle of a two-dimensional dynamical system (the Li'enard system), it can stably perform optimization without imposing explicit constraints on the control parameters. As an illustrative example, we optimize a process in which a fluid contained in a cylindrical vessel is mixed by periodically rotating the vessel. The resulting optimal vessel motion is physically reasonable: it reverses its direction of rotation before a solid-body rotation state is established. Furthermore, even when the fluid viscosity increases with time during the mixing process, the method can continuously adapt the control parameters to the changing viscosity.

physics.flu-dyn↗