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arXiv · 2301.11138

Optical orientation of excitons in a longitudinal magnetic field in indirect band gap (In,Al)As/AlAs quantum dots with type-I band alignment

T. S. Shamirzaev·A. V. Shumilin·D. S. Smirnov·D. Kudlacik·S. V. Nekrasov·Yu. G. Kusrayev·D. R. Yakovlev·M. Bayer
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Abstract

The exciton recombination and spin dynamics in (In,Al)As/AlAs quantum dots (QDs) with indirect band gap and type-I band alignment are studied. The negligible (less than $0.2~\mu$eV) value of the anisotropic exchange interaction in these QDs prevents a mixing of the excitonic basis states with pure spin and allows for the formation of spin polarized bright excitons for quasi-resonant circularly polarized excitation. In a longitudinal magnetic field, the recombination and spin dynamics of the excitons are controlled by the hyperfine interaction between the electron and nuclear spins. A QD blockade by dark excitons is observed in magnetic field eliminating the impact of the nuclear spin fluctuations. A kinetic equation model, which accounts for the population dynamics of the bright and dark exciton states as well as for the spin dynamics, has been developed, which allows for a quantitative description of the experimental data.

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T. S. Shamirzaev, A. V. Shumilin, D. S. Smirnov, D. Kudlacik, S. V. Nekrasov, Yu. G. Kusrayev, D. R. Yakovlev, M. Bayer. 2023-01-26. Optical orientation of excitons in a longitudinal magnetic field in indirect band gap (In,Al)As/AlAs quantum dots with type-I band alignment. https://arxiv.org/abs/2301.11138

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