Search arXivSearch

arXiv · 2401.11996

Elasticity of self-organized frustrated disordered spring networks

Abstract

There have been some interesting recent advances in understanding the notion of mechanical disorder in structural glasses and the statistical mechanics of these systems' low-energy excitations. Here we contribute to these advances by studying a minimal model for structural glasses' elasticity in which the degree of mechanical disorder -- as characterized by recently introduced dimensionless quantifiers -- is readily tunable over a very large range. We comprehensively investigate a number of scaling laws observed for various macro-, meso- and microscopic elastic properties, and rationalize them using scaling arguments. Interestingly, we demonstrate that the model features the universal quartic glassy vibrational density of states as seen in many atomistic and molecular models of structural glasses formed by cooling a melt. The emergence of this universal glassy spectrum highlights the role of self-organization (towards mechanical equilibrium) in its formation, and elucidates why models featuring structural frustration alone do not feature the same universal glassy spectrum. Finally, we discuss relations to existing work in the context of strain-stiffening of elastic networks and of low-energy excitations in structural glasses, in addition to future research directions.

Explore related subjects

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

Tommaso Pettinari, Gustavo Düring, Edan Lerner. 2024-01-22. Elasticity of self-organized frustrated disordered spring networks. https://arxiv.org/abs/2401.11996

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

Deformation and organization of droplet-encapsulated soft beads

Many biological, culinary, and engineering processes lead to the co-encapsulation of several soft particles within a liquid interface. In these situations the particles are bound together by the capillary forces that deform them and influence their biological or rheological properties. Here, we introduce an experimental approach to encapsulate a controlled number of soft beads within aqueous droplets in oil. These droplet-encapsulated gels are manipulated in a deformable microfluidic device to merge them and modify the liquid fraction. In the dry limit the contact surface between the hydrogels is found to be determined by the elastocapillary number $E_c$, with the contact radius following a $E_c^{1/3}$ dependence, indicating that the deformation increases for soft or small particles. When multiple beads are co-encapsulated within a single droplet they can be arranged into linear or three-dimensional aggregates that remain at a local energy minimum.

cond-mat.soft

Flexoelectricity-driven softening of bend elasticity leads to spontaneous chiral symmetry breaking in a polar fluid

The origin of the recently observed spontaneous chiral symmetry breaking in polar fluids composed of achiral molecules is an unsolved problem, raising fundamental questions about how heliconical structures emerge in such systems. Here, we investigate the pretransitional fluctuations leading to the formation of the spontaneously chiral twist-bend ferroelectric nematic phase using dielectric spectroscopy, light scattering, and small-angle X-ray scattering. We observe simultaneous softening of the bend elastic constant and the emergence of a collective dielectric mode on approaching the transition. By developing a theoretical model, we show that these phenomena are signatures of a flexoelectricity-driven transition arising from the coupling between electric polarization and bend deformation.

cond-mat.soft

Taylor dispersion in a soft tube

Diffusion of a solute along a tube is enhanced by hydrodynamic flow, a phenomenon known as Taylor dispersion. In microfluidic applications, the compliance of the tube boundaries modifies the hydrodynamic flow and thus solutal transport. Here, we develop the theory of solutal dispersion in a soft, axisymmetric tube where the tube walls respond to the hydrodynamic pressure through a Winkler response. By deriving the modified macro-transport equation for the solutal concentration dynamics based on multiple-time-scale analysis, we explore the influence of softness on solutal transport for steady and pulsatile configurations. Our main finding is that softness enhances the effective advection velocity and dispersion coefficient, which might have practical implication in biology and microfluidic technology.

cond-mat.soft