Sub-cycle modulation of light's Orbital Angular Momentum

Abstract

The exploration of light has traditionally focused on its spatial properties, particularly its orbital angular momentum (OAM), while its temporal dynamics have remained an underexplored frontier due to the slow response times of existing modulation techniques. In this context, we introduce a method to modulate the OAM of light on a femtosecond scale by engineering a controllable space-time coupling in ultrashort pulses. By intricately linking azimuthal position with time, we implement a static, azimuthally varying wavefront transformation to dynamically alter the spatial distribution of light in a fixed transverse plane. Our experiments demonstrate self-torqued wave packets that exhibit spiraling motions and rapid temporal OAM changes down to a few femtoseconds. We further extend this concept to generate wave packets that angularly self-accelerate. We reveal that these wave packets dynamically adjust their OAM by redistributing their energy density across their spectral bandwidth, all without the influence of external forces. Owing to the unique properties of self-torque and angular acceleration, these time-varying OAM beams offer an accessible avenue for exploring light at fundamental time scales, with far-reaching implications for ultrafast spectroscopy, nano- and micro-structure manipulation, condensed matter physics, and other related areas.