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arXiv · 2406.11212

Low-Energy Electronic Structure in the Unconventional Charge-Ordered State of ScV$_6$Sn$_6$

Asish K. Kundu·Xiong Huang·Eric Seewald·Ethan Ritz·Santanu Pakhira·Shuai Zhang·Dihao Sun·Simon Turkel·Sara Shabani·Turgut Yilmaz·Elio Vescovo·Cory R. Dean·David C. Johnston·Tonica Valla·Turan Birol·Dmitri N. Basov·Rafael M. Fernandes·Abhay N. Pasupathy
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Abstract

Kagome vanadates {\it A}V$_3$Sb$_5$ display unusual low-temperature electronic properties including charge density waves (CDW), whose microscopic origin remains unsettled. Recently, CDW order has been discovered in a new material ScV$_6$Sn$_6$, providing an opportunity to explore whether the onset of CDW leads to unusual electronic properties. Here, we study this question using angle-resolved photoemission spectroscopy (ARPES) and scanning tunneling microscopy (STM). The ARPES measurements show minimal changes to the electronic structure after the onset of CDW. However, STM quasiparticle interference (QPI) measurements show strong dispersing features related to the CDW ordering vectors. A plausible explanation is the presence of a strong momentum-dependent scattering potential peaked at the CDW wavevector, associated with the existence of competing CDW instabilities. Our STM results further indicate that the bands most affected by the CDW are near vHS, analogous to the case of {\it A}V$_3$Sb$_5$ despite very different CDW wavevectors.

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Asish K. Kundu, Xiong Huang, Eric Seewald, Ethan Ritz, Santanu Pakhira, Shuai Zhang, Dihao Sun, Simon Turkel, Sara Shabani, Turgut Yilmaz, Elio Vescovo, Cory R. Dean, David C. Johnston, Tonica Valla, Turan Birol, Dmitri N. Basov, Rafael M. Fernandes, Abhay N. Pasupathy. 2024-06-17. Low-Energy Electronic Structure in the Unconventional Charge-Ordered State of ScV$_6$Sn$_6$. https://doi.org/10.1038/s41467-024-48883-0

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