Magnetic Correlations and Pairing Tendencies of the Hybrid Stacking Nickelate Superlattice La$_7$Ni$_5$O$_{17}$ (La$_3$Ni$_2$O$_7$/La$_4$Ni$_3$O$_{10}$) under Pressure

Abstract

Motivated by the recent rapid progress in high-$T_c$ nickelate superconductors, we comprehensively study the physical properties of the alternating bilayer trilayer stacking nickelate La$_7$Ni$_5$O$_{17}$. The high-symmetry phase of this material, without the tilting of oxygen octahedra, is not stable at ambient conditions but becomes stable under high pressure, where a small hole pocket $\gamma_0$, composed of the $d_{3z^2-r^2}$ states in the trilayer sublattice, appears. This pocket was identified in our previous work for trilayer La$_4$Ni$_3$O$_{10}$ as important to develop superconductivity. Moreover, using random-phase approximation calculations, we find a leading $s^\pm$ pairing state for the high-symmetry phase under pressure with similar pairing strength as that obtained previously for the bilayer La$_3$Ni$_2$O$_7$ compound, suggesting a similar or higher superconducting transition temperature $T_c$. In addition, we find that the dominant magnetic fluctuations in the system driving this pairing state have antiferromagnetic structure both in-plane and between the planes of the top and bottom trilayer and bilayer sublattices, while the middle trilayer is magnetically decoupled.