Distinct amplitude mode dynamics upon resonant and off-resonant excitation across the charge density wave energy gap in LaTe3 investigated by time- and angle-resolved photoemission spectroscopy

Kecheng Liu; Takeshi Suzuki; Yigui Zhong; Teruto Kanai; Jiro Itatani; Linda Ye; Maya Martinez; Anisha Singh; Ian R. Fisher; Uwe Bovensiepen; Kozo Okazaki

doi:10.7566/jpsj.94.104706

arXiv · 2412.13604

Distinct amplitude mode dynamics upon resonant and off-resonant excitation across the charge density wave energy gap in LaTe3 investigated by time- and angle-resolved photoemission spectroscopy

Kecheng Liu·Takeshi Suzuki·Yigui Zhong·Teruto Kanai·Jiro Itatani·Linda Ye·Maya Martinez·Anisha Singh·Ian R. Fisher·Uwe Bovensiepen·Kozo Okazaki

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Abstract

Non-equilibrium states generated by ultrafast laser pulses are characterized by specific phenomena that are not accessible in static measurements. Previous time- and angle-resolved photoemission spectroscopy (TARPES) studies on rare-earth tritelluride materials have revealed the laser-driven melting of the charge density wave order as well as its collective amplitude mode excitation. Variation of the excess energy deposited by optical pumping in the material promises pathways to control the dynamic material response. To this end, we use an optical parametric amplifier to generate a tunable pump photon energy. Studying LaTe3 we compare the dynamics driven by pumping resonantly across the charge density wave energy gap with the effect of pumping at a twice higher photon energy in a TARPES pump-probe experiment. We clearly identify a pump photon energy dependent behavior. At the larger pump photon energy, the excess electronic energy generates lattice heating mediated by e-ph coupling and softening of the amplitude mode frequency from 3 to 2 THz. Remarkably, the resonant pumping across the CDW gap results in a time-independent amplitude mode frequency. We conclude that the resonant excitation across the energy gap excites the amplitude mode selectively while additional electronic excess energy deposited at higher pump photon energy modifies the crystal properties transiently by incoherent dissipative processes.

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Kecheng Liu, Takeshi Suzuki, Yigui Zhong, Teruto Kanai, Jiro Itatani, Linda Ye, Maya Martinez, Anisha Singh, Ian R. Fisher, Uwe Bovensiepen, Kozo Okazaki. 2025-10-17. Distinct amplitude mode dynamics upon resonant and off-resonant excitation across the charge density wave energy gap in LaTe3 investigated by time- and angle-resolved photoemission spectroscopy. https://doi.org/10.7566/jpsj.94.104706

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