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arXiv · 2503.23479

Chiral symmetry and magnetism in a 3D Kagome lattice: RPt$_2$B (R = La and Nd) prototype crystals

C. E. Ardila-Gutiérrez·D. Torres-Amaris·Rafael González-Hernández·Aldo. H. Romero·A. C. Garcia-Castro
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Abstract

Chirality in crystals arises from the exclusive presence of proper symmetry operations, such as rotations and screw axes, while lacking improper operations like inversion, mirror planes, and roto-inversions. Crystallographic chirality is expected to be coupled with magnetic responses in magnetically active chiral compounds. Therefore, this study investigates the interplay between structural chirality and magnetic ordering in the rare-earth platinum boride family, RPt$_2$B, where R denotes lanthanide elements. Our results show that the R sites structurally form a chiral three-dimensional Kagome lattice, which can lead to magnetic frustration resolved through chiral antiferromagnetic orderings in conjunction with chiral symmetry. Symmetry analysis reveals that these chiral antiferromagnetic states are low-energy states, competing with higher-in-energy (001) ferromagnetic configuration. We also identified Kramers-type Weyl points in the electronic structure without magnetic response. In the magnetically active chiral compound NdPt$_2$B, Zeeman splitting lifts degeneracies at the high-symmetry points; however, Weyl points persist due to the breaking of time-reversal (T) and inversion (P) symmetries. We also estimate the anomalous Hall conductivity, a measurable observable of the allowed topological features finding a value of $σ_{xy} = 293$ S$\cdot$cm$^{-1}$ comparable with another Kagome magnetic materials like Mn$_3$PtN and FeSn, for example. This study elucidates the intricate interplay among chirality, magnetism, and topology in rare-earth Kagome materials.

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C. E. Ardila-Gutiérrez, D. Torres-Amaris, Rafael González-Hernández, Aldo. H. Romero, A. C. Garcia-Castro. 2025-03-30. Chiral symmetry and magnetism in a 3D Kagome lattice: RPt$_2$B (R = La and Nd) prototype crystals. https://doi.org/10.1103/w5dn-z87b

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