Search arXivSearch

arXiv · 2508.02395

A comprehensive study of second and third harmonic conversion efficiency, angular and temperature tolerance, and long-term stability in LBO crystals using a 10-J-class laser

Abstract

We present a study of second harmonic generation (SHG) and third harmonic generation (THG) in lithium triborate (LBO) crystals using a high-energy, 10-J-class, 10 Hz Yb:YAG laser system. We achieved high conversion efficiencies of 75% for SHG and 56% for THG for Gaussian-like temporal pulse shapes and top-hat-like beam profiles. The angular and temperature dependence of the LBO crystals were measured and validated through numerical simulations. The SHG process exhibited an angular acceptance bandwidth of 1.33 mrad and a temperature acceptance bandwidth of 2.61 K, while the THG process showed 1.19 mrad and 1.35 K, respectively. Additionally, long term stability measurements revealed RMS energy stabilities of 1.3% for SHG and 1.24% for THG. These results showcase the reliability of LBO crystals for high-energy, high-average-power harmonic generation. The developed system offers automated switching between harmonics provided at the system output. The system can be easily adapted to Nd:YAG based pump lasers as well.

Explore related subjects

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

Huzefa Aliasger, Ondřej Novák, Zbyněk Hubka, Martin Hanuš, Petr Navrátil, Patricie Severová, Ondřej Denk, Jan Pilař, Tomáš Paliesek, Martin Divoký, Ondřej Schreiber, Michal Jelínek, Martin Smrž, Tomáš Mocek. 2025-08-05. A comprehensive study of second and third harmonic conversion efficiency, angular and temperature tolerance, and long-term stability in LBO crystals using a 10-J-class laser. https://doi.org/10.1017/hpl.2025.10067

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

Nonlinear Magneto-Optical Probing of Time-Reversal Symmetry Breaking

Solid-state harmonic generation provides a nonlinear probe of symmetries encoded in electronic wave functions. In the subgap and weak-injection regime, time reversal pairs the harmonic responses driven by fields of opposite ellipticity, strongly suppressing elliptical dichroism in time-reversal-symmetric crystals. We show that, in a magnetic crystal, spin-orbit coupling transfers time-reversal-symmetry breaking from the spin sector to the orbital wave functions and lifts this pairing through the geometric phases of the electric-dipole current. Semiconductor-Bloch-equation calculations for centrosymmetric bilayer Cr2Ge2Te6 predict pronounced third-harmonic elliptical dichroism that reverses with the magnetization. Under linearly polarized driving, SOC-induced geometric-phase accumulation generates a nonlinear transverse current and strongly enhances the harmonic rotation and ellipticity. These results identify the geometric phase as a key microscopic contribution to the nonlinear magneto-optical response. This work establishes helicity-resolved harmonic emission and nonlinear polarimetry as complementary probes of spin-orbit-coupled magnetic order.

physics.optics

Spatiotemporal topological phase transitions in photonic spacetime crystals

Topological phase transitions have played a central role in topological physics. However, such transitions have so far been restricted to spatial or temporal crystals. Here, we transcend this conventional framework and report, for the first time, spatiotemporal topological phase transitions in photonic spacetime crystals - structures that are periodically modulated in both space and time. In a genuine photonic spacetime crystal composed of a dynamically modulated transmission-line metamaterial, we theoretically propose and experimentally demonstrate complete spatiotemporal topological phase transitions, characterized by the closing and reopening of both energy and momentum band gaps, along with changes in spatiotemporal topological invariants and topological phases. Furthermore, we directly observe a spatiotemporal, topologically localized state that exhibits causality-governed excitation and robustness to spatiotemporal disorders. Our findings reveal the interplay among space, time, and topology, establishing a unified framework that provides a comprehensive picture of the emerging topological spacetime physics and opening new avenues for robust spatiotemporal topological wave manipulations.

physics.optics

High-Resolution Sensing via Quantum States Discrimination

High-resolution sensing plays a significant role in scientific research and industrial production, but the practical implementation is constrained by the physical mechanisms of the sensors. To address the critical limitation, we propose a high-resolution sensing approach based on quantum state discrimination. Distinct from conventional strategies, the proposed approach constructs measurement operators in the orthogonal complement space rather than eigenspace of the eigenstate, thereby notably improving the discriminability among quantum states. Moreover, the experimental results via an optical microcavity demonstrate a potential sensing resolution of 4 $\times$ 10\textsuperscript{-6} \degree C and 18 p$ε$ respectively for temperature and strain, and further verify the feasibility of simultaneous sensing of the two parameters. This work establishs a universal approach for high-resolution sensing, and may be extended to different sensing platforms across various application scenarios.

physics.optics