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arXiv · 2509.03022

Aging of glass-forming materials following a temperature jump

Ayata Ueno·Tomoko Mizuguchi·Takashi Odagaki
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Abstract

Physical aging is one of the non-equilibrium phenomena where physical properties change over time due to structural relaxation. Aging in spin glass systems has been explained by a trap model on the temperature-independent energy landscape. Meanwhile, in the free energy landscape (FEL) approach to aging phenomena, it is assumed that the FEL responds to temperature changes with a time delay. In this paper, aging in a glass forming model in which both the trapping effect and the delayed response of the FEL exist is studied after the temperature is changed. It is confirmed that the trapping effect gives rise to Type-I aging where the relaxation time increases with waiting time regardless of the direction of temperature change, and that the delayed response of the FEL produces Type-II aging where the waiting-time dependence of the relaxation time depends on the direction of temperature change. When both effects exist and the response time of the FEL is appropriate, these effects can be differentiated in the short-time behavior of the temporal relaxation time. It is argued that the material time or the internal clock and the fictive temperature introduced phenomenologically are understood as the concepts describing the delayed response of the FEL to temperature change.

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Ayata Ueno, Tomoko Mizuguchi, Takashi Odagaki. 2025-09-05. Aging of glass-forming materials following a temperature jump. https://doi.org/10.1016/j.jnoncrysol.2025.123755

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