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arXiv · 2509.05788

Magnetocrystalline Anisotropy and 3D Hopping Conduction at the Surface of FeSb2

Abstract

Motivated by the recent discovery of metallic surface states in the d-electron Kondo insulator candidates FeSi and FeSb2, along with some recent reports of magnetic correlations in the surface transport properties of FeSi, we have investigated the low temperature surface magnetotransport properties of FeSb2. By using a Corbino disk transport geometry, we were able to isolate the electrical transport properties of a single surface of our samples and study the [110] and [101] naturally forming faces separately. Studying the relationship between the applied magnetic field, current direction and crystal symmetry has allowed us to separate possible contributions to the magnetotransport anisotropy. Unlike previous studies of SmB6 surface states, we find no two-dimensional Drude-like dependence on field orientation relative to current direction, but instead a magnetocrystalline anisotropy that appears to originate from local moment scattering with a well defined easy-axis along the [100] direction. We compare these results with the magnetotransport properties of the conducting surface states on the [111] facet of FeSi. We also find evidence of 3D variable-range hopping conduction below the bulk-to-surface crossover, extending below 1 K, which implies that the electrical transport at the surface of these materials is carried by a thin, but 3D conducting channel, which is inconsistent with the lower dimensional states expected for a strong topological insulator.

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Jarryd A. Horn, Yun Suk Eo, Keenan Avers, Hyeok Yoon, Ryan G. Dorman, Shanta R. Saha, Johnpierre Paglione. 2025-09-06. Magnetocrystalline Anisotropy and 3D Hopping Conduction at the Surface of FeSb2. https://arxiv.org/abs/2509.05788

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