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arXiv · 2512.03833

Shell formation and two-dimensional nanofriction in three-dimensional ion Coulomb crystals

L. -A. Rüffert·T. E. Mehlstäubler
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Abstract

Self-organized three-dimensional (3D) ion Coulomb crystals in linear Paul traps naturally form concentric shells that provide a curved, atomically resolved interface for studying two-dimensional (2D) nanofriction. Building on earlier studies of one-dimensional nanofriction and orientational melting in 2D ion crystals, we extend friction studies from linear chains and planar rings to 3D shell structures. Using molecular-dynamics simulations, we map shell formation as a function of ion number N and trap aspect ratio and obtain a simple scaling relation that can aid ion-number estimation in experiments. We compute a Peierls-Nabarro-type potential for rotating the outer shell against a static inner core, using the rotation angle as a collective coordinate. Changing N by one can alter the effective rotational barrier by up to a factor of ~7, while changes by only a few ions can lead to variations up to a factor of ~60. Combining geometric commensurability analysis with energy decomposition, we show that the barrier is governed by a system-dependent interplay between inter-shell interaction, outer-shell response and trap confinement. Dynamical simulations with applied torques reveal pinned, stick-slip and smooth-sliding regimes with depinning thresholds that depend on ion number, inner-shell geometry and trap aspect ratio. Some configurations show hysteresis due to torque-induced metastable states. We further find that spatially varying coupling to the inner-core corrugation can create coexisting fast and slow domains within the rotating outer shell, realizing multidimensional friction in which intra-shell shear and inter-shell nanofriction act simultaneously. Our results establish self-organized ion Coulomb crystals as model systems for 2D nanofriction and suggest routes toward ion-based nanorotors, torque sensors and ultra-low-friction nanomechanical systems.

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L. -A. Rüffert, T. E. Mehlstäubler. 2026-05-20. Shell formation and two-dimensional nanofriction in three-dimensional ion Coulomb crystals. https://doi.org/10.1103/97sw-7x29

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