Residual Force Determines Surface Tension in Active Systems

Abstract

The mechanical tension at the interface of motility-induced phase separating active Brownian particles (ABPs) remains an open question. Here, we determine the surface tension by analyzing the spatial distribution of forces at the molecular level in a slab-confined system of ABPs exhibiting high and low density regions separated by a one-dimensional active interface. Unlike previous approaches that evaluate active and interaction stresses independently - often producing near-zero or negative surface tension - we show that on average, interaction forces act antagonistically to active propulsion, reducing the net force experienced by particles. By evaluating the work required to bring a particle to the interface using this total-force framework, we find a positive and physically consistent surface tension. These results reframe the mechanical interpretation of local stresses and provide a generalizable method for connecting microscopic force distributions to emergent interfacial properties in nonequilibrium systems.