arXiv · 2512.09698
Contrasting magnetic behavior in MnSc_2X_4 (X = S, Se) spinel compounds investigated by magnetoelastic studies
Abstract
The spinel compounds MnSc_2X_4 are highly frustrated and candidate materials for vortex-like 3q magnetic states, such as skyrmions, with propagation vectors in the [111] plane. Because of the strong magnetoelastic coupling, we could extract a refined magnetic (H, T) phase diagram for MnSc_2S_4 from ultrasound and dilatometry measurements. We found a variety of magnetic phases, including the skyrmion phase, which is stable down to lowest temperatures. In comparison, we investigated MnSc_2Se_4 , having a larger distance between the magnetic Mn^3+ ions using the same methods. Unlike in MnSc_2S_4 , we found no skyrmion phase and overall a lack of sharp anomalies indicative of phase transitions, neither in dilatometry nor ultrasound nor in specific heat and ac-susceptibility data. Motivated by our findings, we performed model calculations, which reproduced the experimentally observed magnetostriction and specific-heat results reasonably well.
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J. Grumbach, J. Sourd, M. Deeb, A. Miyata, H. Suwa, T. Gottschall, A. Hauspurg, S. Chattopadhyay, M. Rotter, S. Granovsky, L. Prodan, V. Tsurkan, S. Zherlitsyn, M. Doerr, J. Wosnitza. 2025-12-10. Contrasting magnetic behavior in MnSc_2X_4 (X = S, Se) spinel compounds investigated by magnetoelastic studies. https://doi.org/10.1103/479d-4jvy
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