Collective Nuclear Polaritons with Coherent and Tunable Excitation Dynamics

Abstract

We propose collective nuclear polaritons formed by hybridizing a 229Th nuclear ensemble with a vacuum-ultraviolet cavity mode generated via four-wave mixing, achieving a collective light-matter coupling that scales as $\sqrt{N}$. In the strong-coupling regime the system displays vacuum Rabi oscillations, indicating the hybridization between cavity photons and nuclear excitations. In the superradiant regime, the stored excitation is released in a cooperative burst with peak intensity scaling as $N^2$. The emission lifetime shrinks from thousands of seconds to the millisecond scale and remains tunable. Detuning sweeps across the polariton avoided crossing allow adiabatic conversion of the photonic excitation into a collective nuclear excitation, enabling reversible quantum storage. Our results demonstrate that cavity-mediated nuclear polaritons enable deterministic lifetime engineering and coherent quantum storage in nuclear systems.