Search arXiv⌕ Search
Home/Archive/arXiv

arXiv · 2604.00991

Excitations across the equilibrium and photoinduced `hidden' states of magnetoresistive manganites

Shiyu Fan·Feng Jin·Taehun Kim·Umesh Kumar·Zixun Zhang·Vivek Bhartiya·Jiemin Li·Brandon Yalin·Yanhong Gu·Mingqiang Gu·Wen Hu·Claudio Mazzoli·G. Lawrence Carr·Osor S. Barišić·Andrey S. Mishchenko·Valentina Bisogni·Sobhit Singh·Wenbin Wu·Jonathan Pelliciari
View original source ↗Read source document ↗Export metadata ↓

Abstract

"Hidden" phases, generated using ultrafast laser pulses (few hundred femtoseconds), with properties distinct from thermodynamic equilibrium, are appealing for technologies because they can be long-lived, with lifetimes of hours or weeks, and reversible with temperature sweeping or extra pulses. In this regard, La$_{2/3}$Ca$_{1/3}$MnO$_3$ (LCMO) stands out due to its tunability through epitaxial strain, which can drive the bulk ferromagnetic metal (FMM) into an antiferromagnetic insulator (AFI), and its susceptibility to photo-induced transitions. Indeed, AFI LCMO displays a long-lived photo-induced transition into a putative 'hidden' phase whose exact nature and excitations are still largely unknown. Here, we combine ultrafast photo-excitation in the near infrared with in situ transport, x-ray absorption (XAS), and Resonant Inelastic X-ray Scattering (RIXS) to investigate the excitations (polarons, phonons, and orbital) of the photo-excited phase of LCMO and contrast them with the thermodynamic phases achieved through strain and temperature. In the thermodynamic regime, we establish the correlation between polarons and transport, placing them in the 'strong coupling' regime of the Holstein model. Upon photo-excitation of LCMO-AFI, we uncover a long-lived phase characterized by the softening of the polaron excitations, the partial suppression of the Jahn-Teller distortion, and nearly unchanged phonons, showing the emergence of a photo-excited state absent in the equilibrium phase diagram. Finally, by varying temperature, epitaxial strain, and photo-excitation fluence, we construct a polaron phase diagram and identify the key spectroscopic signatures of each phase. Our laser-RIXS approach establishes a versatile platform for exploring photo-induced 'hidden' phases in quantum materials in non-stroboscopic conditions.

Explore related subjects

cond-mat.str-el

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

Shiyu Fan, Feng Jin, Taehun Kim, Umesh Kumar, Zixun Zhang, Vivek Bhartiya, Jiemin Li, Brandon Yalin, Yanhong Gu, Mingqiang Gu, Wen Hu, Claudio Mazzoli, G. Lawrence Carr, Osor S. Barišić, Andrey S. Mishchenko, Valentina Bisogni, Sobhit Singh, Wenbin Wu, Jonathan Pelliciari. 2026-04-01. Excitations across the equilibrium and photoinduced `hidden' states of magnetoresistive manganites. https://doi.org/10.1103/24wn-q427

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

arXiv2026

An Exact Conjugation Identity for the Many-Body Wilson Loop Beyond Quantization

Constraints on unquantized many-body holonomies, such as Wilson loops (or their Berry phases), are less explored than those on their quantized counterparts. Here, we realize an unquantized regime by tuning the bond dimerization $δ$ and the staggered potential $Δ$ in a half-filled dimerized staggered Hubbard ring. For the tuned parameter sets, a finite excitation gap persists along the $U(1)$ twist cycle $θ\in[0,2π]$, so that the ground state $|ψ_δ(θ)\rangle$ remains separated from the excited states. The many-body Wilson loop is therefore well defined from the ground-state family $\{|ψ_δ(θ)\rangle;\,θ\in[0,2π]\}$. In this setup, we show an exact many-body Wilson loop conjugation identity, $W(-δ)=W(δ)^*$, accumulated along a cycle parametrized by $θ$. Importantly, the identity persists in regimes where the Berry phase $γ\equiv-\arg W$ varies continuously. We demonstrate the identity numerically using the density-matrix renormalization group (DMRG) method. The identity extends to other models where the flux-threaded ground-state family along the closed $θ$-cycle is mapped to the reversed cycle. Beyond its conceptual content, the identity provides a symmetry-based consistency check for numerical evaluations of Berry phases in interacting systems. It also justifies the signal-to-noise ratio improvement in Monte Carlo simulations by performing simulations at both $δ$ and $-δ$ and averaging $W(δ)$ with $W(-δ)^{*}$.

cond-mat.str-el↗
arXiv2026

Torus Berry Data Determine All-Genus Abelian Topological Orders

We show that for Abelian Chern-Simons topological orders, torus Berry matrices determine the all-genus extended TQFT. We identify the topological part of the projective Berry holonomy under metric deformations with the mapping-class-group representation of the Abelian Chern-Simons TQFT and prove that the normalized torus data reconstruct its finite quadratic module (G,q). Recent work showed that (G,q) classifies the extended theory up to symmetric monoidal natural isomorphism, and that the associated Abelian defect extension is determined by the pointed modular category C(G,q) arising from the same finite quadratic-module data. Therefore genus-one Berry data determine not only the all-genus bulk theory but also its associated defect structures without choosing a K-matrix presentation. We also prove that, for normalized character row errors $δ$<21.96%, nearest-row decoding recovers the Abelian fusion algebra independently of the number of anyons. The result applies to Abelian fractional quantum Hall and spin-liquid phases described by even-lattice Chern-Simons theories.

cond-mat.str-el↗
arXiv2026

Accidental accuracy and vertex corrections in $GW$: Exact benchmarks for the extended Hubbard model

The $GW$ approximation is the standard tool for quasiparticle predictions in materials, yet its regime of validity in correlated systems remains poorly quantified, because \textit{ab initio} vertex corrections are computationally prohibitive. Using exact diagonalization of the half-filled extended Hubbard model on finite rings as a numerically exact reference, we construct the corresponding model-space $GW$ theory on the identical Hilbert space and quantify its error as a function of local ($U$) and non-local ($V$) interaction strength. We find that the required vertex correction changes character across the phase diagram: in the weak-coupling regime the effective vertex $Γ_{\rm eff} < 1$, reflecting the suppression of RPA charge fluctuations by exact short-range correlations, whereas in the Mott regime $Γ_{\rm eff}$ grows monotonically (to $\sim 3$ at $U=8t$ for $N=6$), reflecting the local dynamical self-energy structure required to open the Hubbard gap. Vertex corrections in the electron-hole (polarizability) channel are shown to \emph{worsen} the gap error, indicating that reproducing the Mott gap requires dynamical self-energy structure rather than improved screening. For $V=0$, static COHSEX is accidentally exact at a single crossover $U^* \approx 3.5\,t$; finite $V$, through non-local Fock exchange, splits this point into a double-crossover window that collapses toward weak coupling. Even at the crossover, however, the exact spectral function retains Hubbard-band structure that no static functional reproduces, so gap agreement does not imply functional accuracy. These results yield quantitative diagnostics for the reliability of $GW$ in correlated materials.

cond-mat.str-el↗