Taming Randomness in Random Lasers: Programmable Disorder for Active Control of Random Lasing via Electric-Field-Directed Assembly of Nanowires

Abstract

Random lasing exploits multiple scattering to provide optical feedback without conventional resonant cavities, enabling simplified architectures that are readily integrated into compact photonic platforms such as wearable sensors and lab-on-chip devices. However, the same disorder that enables cavity-free lasing also makes it challenging to control and tune the emission properties. Here, an electrically reconfigurable random-lasing platform based on dielectrophoretic assembly of chaining silver nanowires suspended in a dye gain medium is reported. An applied electric field across patterned quadrupole electrodes induces nanowire chaining and programmable alignment, enabling real-time reconfiguration of the disorder landscape. Based on the electrically driven disorder state transitions, tunable random-lasing characteristics, including reduced lasing thresholds, modulation of emission intensity, and control of the polarization state have been demonstrated. Simulations further indicate that chaining enhances scattering relative to absorption, providing more efficient radiative feedback, and the orientation of the nanowire network governs the polarization dependence of the system. These results establish a route to actively modulate random lasing through controllable disorder and point toward adaptive, reconfigurable photonic light sources and sensing systems.