Search arXivSearch

arXiv · 2606.25628

Bath-modes quantitatively capture the nonlinear microrheology of micellar solutions

Abstract

Active microrheology experiments, in which a probe is driven through a complex fluid, often exhibit nonlinear responses that cannot be captured by generalized Langevin equations. Models that couple the probe to a Gaussian field reproduce such nonlinear effects qualitatively, but their large number of parameters hinders direct comparison with experiments. Here, we restrict these models to a small number of field modes and demonstrate that this reduced description quantitatively reproduces a broad range of active microrheology experiments in a micellar solution using a single set of parameters. We further show that the same framework extends naturally to multi-probe systems, such as colloidal dumbbells.

Explore related subjects

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

Pierre Champagnac, Clemens Bechinger, Juliana Caspers, Pierre Illien, Matthias Krüger, Vincent Démery. 2026-06-24. Bath-modes quantitatively capture the nonlinear microrheology of micellar solutions. https://arxiv.org/abs/2606.25628

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

Deformation and organization of droplet-encapsulated soft beads

Many biological, culinary, and engineering processes lead to the co-encapsulation of several soft particles within a liquid interface. In these situations the particles are bound together by the capillary forces that deform them and influence their biological or rheological properties. Here, we introduce an experimental approach to encapsulate a controlled number of soft beads within aqueous droplets in oil. These droplet-encapsulated gels are manipulated in a deformable microfluidic device to merge them and modify the liquid fraction. In the dry limit the contact surface between the hydrogels is found to be determined by the elastocapillary number $E_c$, with the contact radius following a $E_c^{1/3}$ dependence, indicating that the deformation increases for soft or small particles. When multiple beads are co-encapsulated within a single droplet they can be arranged into linear or three-dimensional aggregates that remain at a local energy minimum.

cond-mat.soft

Flexoelectricity-driven softening of bend elasticity leads to spontaneous chiral symmetry breaking in a polar fluid

The origin of the recently observed spontaneous chiral symmetry breaking in polar fluids composed of achiral molecules is an unsolved problem, raising fundamental questions about how heliconical structures emerge in such systems. Here, we investigate the pretransitional fluctuations leading to the formation of the spontaneously chiral twist-bend ferroelectric nematic phase using dielectric spectroscopy, light scattering, and small-angle X-ray scattering. We observe simultaneous softening of the bend elastic constant and the emergence of a collective dielectric mode on approaching the transition. By developing a theoretical model, we show that these phenomena are signatures of a flexoelectricity-driven transition arising from the coupling between electric polarization and bend deformation.

cond-mat.soft

Taylor dispersion in a soft tube

Diffusion of a solute along a tube is enhanced by hydrodynamic flow, a phenomenon known as Taylor dispersion. In microfluidic applications, the compliance of the tube boundaries modifies the hydrodynamic flow and thus solutal transport. Here, we develop the theory of solutal dispersion in a soft, axisymmetric tube where the tube walls respond to the hydrodynamic pressure through a Winkler response. By deriving the modified macro-transport equation for the solutal concentration dynamics based on multiple-time-scale analysis, we explore the influence of softness on solutal transport for steady and pulsatile configurations. Our main finding is that softness enhances the effective advection velocity and dispersion coefficient, which might have practical implication in biology and microfluidic technology.

cond-mat.soft