Few-cycle electro-optic light on thin-film lithium niobate

Abstract

The twin fields of ultrafast optics and nonlinear photonics enable applications ranging from attosecond science [1, 2] and ultrafast electronics [3] to molecular spectroscopy [4, 5], nonlinear optics [6-8], quantum nanophotonics [9] and precision metrology [10]. However, bringing these capabilities-including ultrashort pulse generation, dispersion control, and strong nonlinear interactions-together within a scalable photonic integrated platform requires exceptional performance and cooperation between components while preserving sufficient optical power across the circuit. Here we demonstrate an integrated multi-functional nonlinear photonic system that transforms continuous-wave (CW) light into high-peak-power femtosecond pulses and harnesses them for pulse-driven nonlinear optics on thin-film lithium niobate (TFLN). Microwave-driven electro-optic (EO) broadening followed by integrated dispersive compression generates 230-fs Fourier-transform-limited pulses with energies up to 3.3 pJ at 30.7 GHz, representing orders of magnitude higher pulse energy than previous integrated pulse synthesis at comparable repetition rates [11]. In a 0.3-meter dispersion-engineered TFLN waveguide, soliton dynamics compress the pulses to 35 fs (6.7 optical cycles), accompanied by coherent spectral broadening exceeding 330 nm. In a fully-monolithic architecture, EO synthesis, dispersive compression and a high-Q nonlinear resonator are integrated on a single TFLN chip, enabling resonantly-enhanced pulse pumping and coherent spectral broadening at pulse energies as low as 400 fJ. By unifying microwave-controlled pulse synthesis and pulse-driven nonlinear interactions, our work establishes a direct path from CW excitation to few-cycle nonlinear optics on chip, with opportunities spanning microwave photonics [12], optical frequency synthesis and metrology, and mid-infrared and terahertz generation [13, 14].