Twist-Reconfigurable van der Waals Moiré Photonic Crystals

Abstract

Moiré photonics has emerged as a fascinating concept to design and in situ control of the optical bands. Moiré enabled light localisation arises from the relative twist between periodic layers, rather than from fixed, pre-fabricated cavity features. So far, however, the realisation of practical moiré photonic crystals in the visible range has been elusive, due to challenges in engineering nanoscale structures and twisting them dynamically post fabrication. Here, we realise a mechanically reconfigurable moiré photonic crystal, comprising from two patterned van der Waals crystals (tungsten di sulphide, WS$_2$) slabs separated by an optically active hexagonal boron nitride (hBN) spacer. We reconfigured the same pair of WS$_2$ slabs from a twist angle of 3.8° to 8.4° and reconstructed their three-dimensional dispersion using momentum-resolved reflectivity spectroscopy. Further, by reducing the twist angle between the slabs, we observe a denser manifold of folded and hybridised resonances that coincides with a 30-fold enhancement of emission from embedded colour centres. Our results open exciting opportunities for in-situ dispersion engineering and programmable light matter interactions employing van der Waals nanostructures.