Peeling threshold for removal of an adhered elastic sheet by a shear flow

Abstract

Fluid shear can induce detachment of a thin elastic sheet adhered to a flat substrate. This peeling process is important in a variety of environmental and technological systems. The condition for peeling depends on: the shear rate $\dotγ$, the fluid viscosity $η$, the length of the detached portion of the sheet $L$, the bending rigidity $B$ and the adhesion energy $Γ$. What are the laws governing the detachment? We address this question experimentally in the regime of intermediate adhesion, using macroscopic sheets bonded to a substrate and immersed in a shear cell containing a viscous fluid. The experiments indicate a critical shear rate for peeling of the order of $\dotγ \sim B/(ηL^3)$. This threshold is, unexpectedly, independent of adhesion. We rationalise this result by applying Griffith's fracture theory to optical measurement data of the shape of the sheet, under conditions of freely moving peeling front or clamped boundary. The results indicate that the large curvature of the sheet for $\dotγ \sim B/(ηL^3)$ yields a nearly diverging strain energy release rate at this threshold. This approximate divergence in turn yields a peeling threshold that depends at most weakly on $Γ$, confirming a theory that was proposed recently (Salussolia et al., J. Mech. Phys. Solids, 2020, 134). Among other applications, our work provides a quantitative formula that can aid the production at scale of 2D materials such as graphene.