Classification of fission modes in $^{236}$U using a six-dimensional Langevin approach

Abstract

Thermal neutron-induced fission of $^{235}$U is studied using a six-dimensional Langevin approach based on the Cassini shape parametrization. Scission events are classified into Asymmetric 1 (AS1), Asymmetric 2 (AS2), and Superlong (SL) fission modes by applying the $k$-means algorithm to the fragment mass and the quadrupole deformations of both fragments. For each mode, proton and neutron single-particle levels are calculated for representative fragments to examine their shell structures. The AS1 heavy fragment exhibits proton gaps at $Z=50$ and 52 and neutron gaps at $N=82$ and 84, whereas well-developed gaps appear at $Z=56$ and $N=88$ in the AS2 heavy fragment. The mass splits of AS1 and AS2 are close to those of the conventional Standard I and Standard II modes, respectively. However, the average total kinetic energy is lower for AS1 than for AS2, opposite to the conventional ordering of Standard I and Standard II. This reversal reflects the more elongated shape of the AS1 light fragment. The SL mode is conventionally interpreted in terms of macroscopic liquid-drop effects, whereas the pronounced proton shell gap at $Z=46$ suggests that proton shell effects also contribute to the elongated symmetric configuration. The classification based on fragment mass and the quadrupole deformations of both fragments provides a basis for distinguishing fission modes and examining the corresponding fragment shell structures at scission.