Attosecond topological interference beyond Floquet-Volkov paths

Hyosub Park; J. D. Lee

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arXiv · 2609.30282

Attosecond topological interference beyond Floquet-Volkov paths

Hyosub Park·J. D. Lee

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Abstract

Combining attosecond science with semiconductor physics provides a promising interdisciplinary platform for the attosecond control of semiconducting properties. In each field, the reconstruction of attosecond beating by interference of two-photon transitions (RABBIT) and the time-resolved and angle-resolved photoemission spectroscopy (tr-ARPES) have been central experimental techniques for probing microscopic dynamics of electrons. However, the integration of the two techniques, bridging the two fields, has been missing so far although they have many technical similarities. Here, we develop a theoretical framework that integrates the two techniques based on the second-order time-dependent perturbation theory. Within this framework, we investigate the RABBIT spectroscopy in semiconductors focusing on the recent hallmark of tr-ARPES, namely quantum path interference between Floquet and Volkov states. Moreover, we theoretically identify a novel quantum path incorporating the virtual excitation, which substantially interferes with the Floquet and Volkov states in both the RABBIT spectroscopy and tr-ARPES of semiconductors. Importantly, we find that such virtual excitation channel induces an attosecond topological interference with the Floquet-Volkov paths, encoding topological quantities such as the local Berry curvature into the time shift of RABBIT sidebands, which is directly related to the photoelectron emission delay. Our findings establish a theoretical framework connecting attosecond spectroscopy to tr-ARPES, paving the way for future applications of attosecond science in semiconductors.

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Hyosub Park, J. D. Lee. 2026-08-31. Attosecond topological interference beyond Floquet-Volkov paths. https://arxiv.org/abs/2609.30282

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