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Magnetic structures of RbCuCl_3 in a transverse field

A. E. Jacobs·T. Nikuni
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Abstract

A recent high-field magnetization experiment found a phase transition of unknown character in the layered, frustrated antiferromagnet RbCuCl_3, in a transverse field (in the layers). Motivated by these results, we have examined the magnetic structures predicted by a model of RbCuCl_3, using the classical approximation. At small fields, we obtain the structure already known to be optimal, an incommensurate (IC) spiral with wave vector q in the layers. At higher fields, we find a staircase of long-period commensurate (C) phases (separated initially by the low-field IC phase), then two narrow IC phases, then a fourth IC phase (also with intermediate C phases), and finally the ferromagnetically aligned phase at the saturation field H_S. The three-sublattice C states familiar from the theory of the triangular antiferromagnet are never optimal. The C phases and the two intermediate IC phases were previously unknown in this context. The magnetization is discontinuous at a field \approx 0.4H_S, in qualitative agreement with experiment, though we find much fine structure not reported.

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A. E. Jacobs, T. Nikuni. 2001-11-08. Magnetic structures of RbCuCl_3 in a transverse field. https://doi.org/10.1103/physrevb.65.174405

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