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First Order Transition in the Spin Dynamics of Geometrically Frustrated Yb2Ti2O7

J. A. Hodges·P. Bonville·A. Forget·A. Yaouanc·P. Dalmas de Reotier·G. Andre·M. Rams·K. Krolas·C. Ritter·P. C. M. Gubbens·C. T. Kaiser·P. J. C. King·C. Baines
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Abstract

Using neutron diffraction, 170Yb Mossbauer and muSR spectroscopies, we have examined the pyrochlore Yb2Ti2O7 where the Yb3+ S'=1/2 ground state has planar anisotropy. Below ~0.24K, the temperature of the known specific heat lambda transition, there is no long range magnetic order. We show that the transition corresponds to a first order change in the fluctuation rate of the Yb3+ spins. Above the transition temperature, the rate, in the GHz range, follows a thermal excitation law, whereas below, the rate, in the MHz range, is essentially temperature independent indicative of a quantum fluctuation regime.

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J. A. Hodges, P. Bonville, A. Forget, A. Yaouanc, P. Dalmas de Reotier, G. Andre, M. Rams, K. Krolas, C. Ritter, P. C. M. Gubbens, C. T. Kaiser, P. J. C. King, C. Baines. 2002-01-11. First Order Transition in the Spin Dynamics of Geometrically Frustrated Yb2Ti2O7. https://doi.org/10.1103/physrevlett.88.077204

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